基本信息
亓良  男    中国科学院大连化学物理研究所
电子邮件: qlyanfei920@dicp.ac.cn
通信地址: 大连市中山区457号
邮政编码:

研究领域

    分子筛及金属-分子筛催化是现代能源催化领域的重要基石,分子筛催化理论的持续革新已经为烯烃、芳烃及含氧化合物等重要大宗化学品的生产技术带来多次革命性突破。我们拟围绕分子筛特定T位点(酸中心)利用,分子筛载体上金属位点定向构筑,特定金属位点-酸中心协同催化,结合活性位点的落位和结构解析、反应动力学研究,系统考察分子筛体系催化新C-C键定向生成机制,结合所在团队在分子筛材料领域设计合成的巨大优势,建立科学的分子筛催化C-C键定向生成理论体系,预测并设计新催化反应、开发新催化工艺,形成完整的分子筛催化C-C键定向生成技术路线图。


招生信息

   
招生专业
081705-工业催化
招生方向
分子筛及金属-分子筛催化C-C键定向生成

教育背景

2011-09--2017-07   中国科学院大学大连化学物理研究所   工学博士
2007-09--2011-06   中国石油大学(华东)   本科
学历
工学博士

学位
工学博士

工作经历

   
工作简历
2019-03~2022-03,美国加州大学伯克利分校, 访问学者
2017-09~现在, 中国科学院大连化学物理研究所, 副研究员
2017-07~2017-09,中国科学院大连化学物理研究所, 助理研究员

专利与奖励

   
专利成果
[1] 王莹利, 亓良, 明政, 郑传龙, 刘中民. 改性ZSM-5分子筛催化剂制备方法及其应用、煤基乙醇制乙烯方法. CN: CN111250150A, 2020-06-09.

出版信息

   
发表论文
[1] Qi, Liang, Das, Sonali, Zhang, Yanfei, Nozik, Danna, Gates, Bruce C, Bell, Alexis T. Ethene Hydroformylation Catalyzed by Rhodium Dispersed with Zinc or Cobalt in Silanol Nests of Dealuminated Zeolite Beta. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY. 2023, [2] Zhang, Yanfei, Qi, Liang, Leonhardt, Branden, Bell, Alexis T. Mechanism and Kinetics of n-Butane Dehydrogenation to 1,3-Butadiene Catalyzed by Isolated Pt Sites Grafted onto SiOZn-OH Nests in Dealuminated Zeolite Beta. ACS CATALYSIS[J]. 2022, 12(6): 3333-3345, http://dx.doi.org/10.1021/acscatal.2c00059.
[3] 刘荣升, 樊本汉, 张雯娜, 王林英, 亓良, 王莹利, 徐舒涛, 于政锡, 魏迎旭, 刘中民. Increasing the Number of Aluminum Atoms in T3 Sites of a Mordenite Zeolite by Low-Pressure SiCl4 Treatment to Catalyze Dimethyl Ether Carbonylation. Angewandte Chemie International Edition[J]. 2022, 134(18): https://onlinelibrary.wiley.com/doi/epdf/10.1002/anie.202116990.
[4] Qi, Liang, Zhang, Yanfei, Babucci, Melike, Chen, Cailing, Lu, Peng, Li, Jingwei, Dun, Chaochao, Hoffman, Adam S, Urban, Jeffrey J, Tsapatsis, Michael, Bare, Simon R, Han, Yu, Gates, Bruce C, Bell, Alexis T. Dehydrogenation of Propane and n-Butane Catalyzed by Isolated PtZn4 Sites Supported on Self-Pillared Zeolite Pentasil Nanosheets. ACS CATALYSIS[J]. 2022, 12(18): 11177-11189, [5] Zhang, Yanfei, Qi, Liang, Lund, Alicia, Lu, Peng, Bell, Alexis T. Mechanism and Kinetics of Acetone Conversion to Isobutene over Isolated Hf Sites Grafted to Silicalite-1 and SiO2. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2021, 143(22): 8352-8366, http://dx.doi.org/10.1021/jacs.1c01315.
[6] Qi, Liang, Babucci, Melike, Zhang, Yanfei, Lund, Alicia, Liu, Lingmei, Li, Jingwei, Chen, Yizhen, Hoffman, Adam S, Bare, Simon R, Han, Yu, Gates, Bruce C, Bell, Alexis T. Propane Dehydrogenation Catalyzed by Isolated Pt Atoms in SiOZn-OH Nests in Dealuminated Zeolite Beta. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2021, 143(50): 21364-21378, http://dx.doi.org/10.1021/jacs.1c10261.
[7] Qi, Liang, Zhang, Yanfei, Conrad, Matthew A, Russell, Christopher K, Miller, Jeffrey, Bell, Alexis T. Ethanol Conversion to Butadiene over Isolated Zinc and Yttrium Sites Grafted onto Dealuminated Beta Zeolite. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY[J]. 2020, 142(34): 14674-14687, https://www.webofscience.com/wos/woscc/full-record/WOS:000566667700030.
[8] 亓良, 李金哲, 王林英, 王婵, 许磊, 刘中民. Comparative investigation of the deactivation behaviors over HZSM-5 and HSAPO-34 catalysts during low-temperature methanol conversion. CATALYSIS SCIENCE & TECHNOLOGY[J]. 2017, 7(10): 2022-2031, https://www.webofscience.com/wos/woscc/full-record/WOS:000401907700007.
[9] Zhou, You, Qi, Liang, Wei, Yingxu, Liu, Zhongmin. Comparative investigation of the MTH induction reaction over HZSM-5 and HSAPO-34 catalysts. MOLECULAR CATALYSIS[J]. 2017, 433: 20-27, http://dx.doi.org/10.1016/j.mcat.2017.02.018.
[10] 亓良, 李金哲, 王林英, 许磊, 刘中民. Unusual deactivation of HZSM-5 zeolite in the methanol to hydrocarbon reaction. CATALYSIS SCIENCE & TECHNOLOGY[J]. 2017, 7(4): 894-901, http://cas-ir.dicp.ac.cn/handle/321008/169492.
[11] Qi, Liang, Li, Jinzhe, Xu, Lei, Liu, Zhongmin. Evolution of the reaction mechanism during the MTH induction period over the 2-dimensional FER zeolite. RSC ADVANCES[J]. 2016, 6(61): 56698-56704, http://cas-ir.dicp.ac.cn/handle/321008/170520.
[12] 周游, 亓良, 魏迎旭, 袁翠峪, 张默之, 刘中民. SAPO-34催化剂上甲醇制烯烃诱导期反应. 催化学报[J]. 2016, 37(9): 1496-1501, http://lib.cqvip.com/Qikan/Article/Detail?id=670308803.
[13] You Zhou, Liang Qi, Yingxu Wei, Cuiyu Yuan, Mozhi Zhang, Zhongmin Liu. Methanol-to-olefin induction reaction over SAPO-34. CHINESE JOURNAL OF CATALYSIS[J]. 2016, 37(9): 1496-1501, http://www.corc.org.cn/handle/1471x/2375784.
[14] Qi, Liang, Li, Jinzhe, Wei, Yingxu, Xu, Lei, Liu, Zhongmin. Role of naphthalene during the induction period of methanol conversion on HZSM-5 zeolite. CATALYSIS SCIENCE & TECHNOLOGY[J]. 2016, 6(11): 3737-3744, http://cas-ir.dicp.ac.cn/handle/321008/170512.
[15] Zhou, You, Qi, Liang, Wei, Yingxu, Yuan, Cuiyu, Zhang, Mozhi, Liu, Zhongmin. Methanol-to-olefin induction reaction over SAPO-34. CHINESE JOURNAL OF CATALYSIS[J]. 2016, 37(9): 1496-1501, http://cas-ir.dicp.ac.cn/handle/321008/170142.
[16] Qi, Liang, Li, Jinzhe, Wei, Yingxu, He, Yanli, Xu, Lei, Liu, Zhongmin. Influence of acid site density on the three-staged MTH induction reaction over HZSM-5 zeolite. RSC ADVANCES[J]. 2016, 6(57): 52284-52291, http://www.corc.org.cn/handle/1471x/2375666.
[17] Qi, Liang, Wei, Yingxu, Xu, Lei, Liu, Zhongmin. Reaction Behaviors and Kinetics during Induction Period of Methanol Conversion on HZSM-5 Zeolite. ACS CATALYSIS[J]. 2015, 5(7): 3973-3982, http://cas-ir.dicp.ac.cn/handle/321008/146397.
[18] 亓良. 甲醇转化为烃类反应诱导期的研究. 

科研活动

   
科研项目
( 1 ) 中国科学院青年促进会人才项目, 负责人, 中国科学院计划, 2023-01--2025-12
参与会议
(1)Propane and Butane Dehydrogenation Catalyzed by isolated PtZn4 site supported over Self-Pillared Zeolite Nanosheets    2022年北美催化会   2022-05-22
(2)Creation of Isolated Pt Atoms in ≡SiOZn-OH Nests in Dealuminated Zeolite Beta for Propane Dehydrogenation   2021年美国化学工程师年会   2021-11-07
(3)Ethanol Conversion to Butadiene over Isolated Zinc and Yttrium Sites in Dealuminated Beta Zeolite   2020年美国化学工程师年会   2020-11-16
(4)Ethanol Conversion to Butadiene over Isolated Zinc and Yttrium Sites in Dealuminated Beta Zeolite   2020年美国化学会秋季年会   2020-08-17