电催化材料数据库的智能设计与高通量筛选

亚稳态电催化材料在小分子介导能量转化中的应用

2012-06--2017-09   吉林大学   工学博士
2008-06--2012-09   烟台大学   工学学士

2024.05--至今, 中国科学院大连化学物理研究所，研究员

2022.11--2024.01, 波鸿鲁尔大学 (Ruhr-Universität Bochum, 德国), 助理研究员

2022.06--2022.10, Dioxycle (法国)，工程师

2019.05--2022.05, 国家科学研究中心（Centre national de la recherche scientifique，CNRS，法国), 博士后

2017.06--2019.04, 蒙纳士大学(Monash University，澳大利亚), 博士后

8. Voiry, D., Qi, K. Process and use of copper based electrocatalyst material in supersaturated electrolyte, EP4209619A1 (European patent)

7. Voiry, D., Qi, K. Electrocatalytic material comprising nitrogen-rich carbon nanosheets with inclusions of metal atoms and use thereof, EP3995603A1 (European patent)

6. Voiry, D., Wu, H. L., Qi, K. Functionalized silver-copper catalysts for electrochemical conversion of CO₂ to small molecules, EP4001470A1 (European patent)

5. Cui, X. Q., Qi, K., Liu, C., Jin, Z. & Liu, L. L. Electro-catalysis hydrogen production material and method for preparing same, AU2021102039A4 (Australian patent)

4. Cui, X. Q., Qi, K., Liu, C., Jin, Z. & Liu, L. L. An electrocatalytic hydrogen production material and its preparation method, ZL201610702660.3 (Chinese patent)

3. Zhang, Y. P., Qi, K. & Bao, Q. L. A trimetallic nanoscale Prussian blue-like material and its applications, ZL201711310285.9 (Chinese patent)

2. Qi, K., Zhang, Y. P. & Bao, Q. L. Gold nanoparticle-modified ITO in electrocatalytic oxidation of ethanol, ZL201810716916.5 (Chinese patent)

1. Cui, X. Q., Qi, K., Zhang, L., Liu, C. & Zhang, H. Y. A molybdenum disulfide nanostructured material and its applications, ZL201710050428.0 (Chinese patent)

2024:

44. Zhang, Y., Qi, K.,* Lyu, P. B., Petit, E., Wu, H. L., Wang, W. S., Ma, J. Y., Wang, Y., S, C. & Voiry, D.* Grain-boundary engineering boosted undercoordinated active sites for scalable conversion of CO₂ to ethylene. ACS Nano, 2024, 10.1021/acsnano.3c12662

43. Wu, H. L., Huang, L. Q., Timoshenko, J., Qi, K., Wang, W. S., Liu, J. F., Zhang, Y., Yang, S. K., Petit, E., Flaud, V., Li, J., Salameh, C., Miele, P., Lajaunie, L., Cuenya, B. R., Rao, D. W.* & Voiry, D.* Selective and energy-efficient electrosynthesis of ethylene from CO₂ by tuning the valence of Cu catalysts through aryl diazonium functionalization. Nature Energy, 2024, 18, 2108316.

2023:

42. Qi, K., Zhang, Y., Onofrio, N., Petit, E., Cui, X. Q., Ma, J. Y., Fan, J. C., Wu, H. L., Wang, W. S., Li, J., Liu, J. F., Zhang, Y. P., Wang, Y., Jia, G. R., Wu, J. D., Lajaunie, L., Salameh, C. & Voiry, D.* Unlocking direct CO₂ electrolysis to C₃ products via electrolyte supersaturation. Nature Catalysis, 2023, 6, 319-331.

41. Wu, H. L.,^# Amrita, S. M.,^# Qi, K.,^# Zeng, Z. Y., Mougel, V.* & Voiry, D.* Electrocatalyst microenvironment engineering for enhanced product selectivity in carbon dioxide and nitrogen reduction reactions. ACS Catalysis, 2023, 13, 8, 5375-5396.

40. Ren, F. H.,^# Qi, K.,^# Liu, J. F., Huguet, P., Voiry, D.* & Deabate, S.* Converting the liquid electrolyte of Li batteries into a catalyst for CO₂RR via laser irradiation. ACS Applied Energy Materials, 2023, 6, 12, 6773-6780.

39. Wang, W. S., Onofrio, N., Petit, E., Karamoko, B. A., Wu, H. L., Liu, J. F., Li, J., Qi, K., Zhang, Y., Gervais, C., Lajaunie, L., Salameh, C., Miele, P., Zeng, Z. Y. & Voiry, D.* High surface area functionalized nanolaminated membranes for energy efficient nanofiltration and desalination in forwards osmosis. Nature Water, 2023, 1, 187-197.

38. Zhou, M., Wang, Z. Q., Mei, A. H., Yang, Z. F., Chen, W., Ou, S. Y., Wang, S. Y.,* Chen, K. Q.,* Reiss, P.,* Qi, K., Ma, J. Y. & Liu Y. L.* Photocatalytic CO₂ reduction using La-Ni bimetallic sites within a covalent organic framework. Nature Communications, 2023, 14, 2473.

37. Li, Z. P., Ma, X. Z.,* Wei, F. X., Wang, D. P., Deng, Z. Y., Jiang, M. T., Siddiquee, A., Qi, K., Zhu, D., Zhao, M., Shen, M. Z., Canepa, P., Kou, S. S., Lin, J.* & Wang, Q.* As-grown miniaturized true zero-order waveplates based on low-dimensional ferrocene crystals. Advanced Materials, 10.1002/adma.202302468.

2022:

36. Li, J., Zhang, Y., Liu, C., Zheng, L. R., Petit, E., Qi, K., Zhang, Y., Wu, H. L., Wang, W. S., Tiberj, A., Wang, X. C., Chhowalla, M., Lajaunie, L., Yu, R. H. & Voiry, D.* 3.4% solar-to-ammonia efficiency from nitrate using Fe single-atom catalyst supported on MoS₂ nanosheets. Advanced Functional Materials, 2022, 18, 2108316.

2021:

35. Qi, K.,^# Zhang, Y.,^# Li, J., Charmette, C., Ramonda, M., Cui, X. Q., Wang, Y., Zhang, Y. P., Wu, H. L., Wang, W. S., Zhang, X. L. & Voiry, D.* Enhancing the CO₂‑to-CO conversion from 2D silver nanoprisms via superstructure assembly. ACS Nano, 2021, 15, 4, 7682-7693.

34. Chen, K. Q.,^# Qi, K.,^# Zhou, T.,^# Yang, T. Q.,^# Zhang, Y. P.,* Guo, Z. N., Xie, Z. J., Lim, C. K., Zhang, B., Ni, X., Zhang, J. Y., Zutic, I., Zhang, H.* & Prasad, P. N.* Water-dispersible CsPbBr₃ perovskites nanocrystals with ultra-stability and its application in electrochemical CO₂ reduction. Nano-Micro Letters, 2021, 11, 102.

33. Wu, H. L., Li, J., Qi, K., Zhang, Y., Petit, E., Wang, W. S., Flaud, V., Onofrio, N., Rebiere, B., Huang, L. Q., Salameh, C., Lajaunie, L., Miele, P. & Voiry, D.* Improved electrochemical conversion of CO₂ to multicarbon products by using molecular doping. Nature Communications, 2021, 12, 7210.

32. Zhang, Y., Qi, K., Li, J., Karamoko, B. A., Lajaunie, L., Godiard, F., Oliviero, E., Cui, X. Q., Wang, Y., Zhang, Y. P., Wu, H. L., Wang, W. S. & Voiry, D.* 2.6% cm^-2 single-pass CO₂-to-CO conversion using Ni single atoms supported on ultra-thin carbon nanosheets in a flow electrolyzer. ACS Catalysis, 2021, 11, 12701-12711.

31. Zhang, Z. Y.,* Zhang, M. Y., Zhang, P. & Qi, K. Smart design, controllable synthesis, and functional applications of low-dimensional hetero-structure materials. Journal of Nanomaterials, 2021, 2021, 9823748.

2020:

30. Qi, K., Chhowalla, M. & Voiry, D.* Single-atom is not alone: Metal-support interactions in single-atom catalysis. Materials Today, 2020, 40, 173-192.

29. Maachou, L.,^# Qi, K.,^# Petit, E., Qin, Z. D., Zhang, Y., Cot, D., Flaud, V., Reibel, C., Maghrbi, E. I., Li, L., Miele, P., Kaplan, D., Chhowalla, M., Onofrio, N. & Voiry, D.* Biomimetic electro-oxidation of alkyl sulfides from exfoliated molybdenum disulfide nanosheets. Journal of Materials Chemistry A, 2020, 8, 25053-25060.

28. Wang Y. D., Wang, Y. W., Chen, K. Q., Qi, K., Xue, T. Y., Zhang, H., He, J.* & Xiao, S.* Niobium carbide MXenes with broad-band nonlinear optical response and ultrafast carrier dynamics. ACS Nano, 2020, 14, 8, 10492-10502.

27. Chen K. Q., Wang, C., Peng, Z. Y., Qi, K., Guo, Z. N., Zhang, Y. P.* & Zhang, H.* The chemistry of colloidal semiconductor nanocrystals: From metal-chalcogenides to emerging perovskite. Coordination Chemistry Reviews, 2020, 418, 1, 213333.

2019:

26. Qi, K., Cui, X. Q.,* Gu, L., Yu, S. S., Fan, X. F., Luo, M. C., Xu, S., Li, N. B., Zheng, L. R., Zhang, Q. H., Ma, J. Y., Gong, Y., Lv, F., Wang, K., Huang, H. H., Zhang, W., Guo, S. J.,* Zheng, W. T.* & Liu, P. Single-atom cobalt array bound to distorted 1T MoS₂ with ensemble effect for hydrogen evolution catalysis. Nature Communications, 2019, 10, 5231.

25. Wang, Y,^# Qi, K.,^# Yu, S. S., Jia, G. R., Cheng, Z. L., Zheng, L. R., Wu, Q., Bao, Q. L. Wang, Q. Q., Zhao, J. X.,* Cui, X. Q.* & Zheng, W. T. Revealing the intrinsic peroxidase-like catalytic mechanism of heterogeneous single-atom Co-MoS₂. Nano-Micro Letters, 2019, 11, 102.

24. Xue, T. Y.,^# Qi, K.^# & Hu, C. Q.* Novel SPR sensing platform based on superstructure MoS₂ nanosheets for ultrasensitive detection of mercury ion. Sensors and Actuators B: Chemical, 2019, 284, 589-594.

23. Liu, L. L., Sun Y. H., Cui, X. Q.,* Qi, K., He, X., Bao, Q. L., Ma, W. L., Lu, J., Fang, H. Y., Zhang, P., Zheng, L. R., Yu, L. P., Singh, D. J., Xiong, Q. H., Zhang, L. J.* & Zheng, W. T.* Bottom-up growth of homogeneous Moiré superlattice in bismuth oxychloride spiral nanosheets. Nature Communications, 2019, 10, 4472.

22. Xue, T. Y., Liang, W. Y., Li, Y. W., Sun, Y. H., Xiang, Y. J., Zhang, Y. P., Dai, Z. G., Duo, Y. H., Wu, L. M., Qi, K., Shivananju, B. N., Zhang, L. J.,* Cui, X. Q.,* Zhang, H.* & Bao, Q. L.* Ultrasensitive detection of miRNA with an antimonene-based surface plasmon resonance sensor. Nature Communications, 2019, 10, 28.

21. Fan, J. C., Cui, X. Q.,* Yu, S. S., Gu, L., Zhang, Q. H., Meng, F. Q., Peng, Z. Q., Ma, L. P., Ma, J. Y., Qi, K., Bao, Q. L. & Zheng, W. T. Interstitial hydrogen atom modulation to boost hydrogen evolution in Pd-based alloy nanoparticles. ACS Nano, 2019, 13, 11, 12987-12995.

20. Shang B., Cui, X. Q.,* Jiao, L., Qi, K., Wang, Y. W., Fan, J. C., Yue, Y. Y., Wang, H. Y., Bao, Q. L., Fan, X. F., Wei, S. T., Song, W., Cheng, Z. L., Guo, S. J. & Zheng, W. T.* Lattice-mismatch-induced ultrastable 1T-phase MoS₂-Pd/Au for plasmon-enhanced hydrogen evolution. Nano Letters, 2019, 19, 5, 2758-2764.

19. Li, X. Z., Fang, Y. Y., Wang, J., Wei, B., Qi, K., Hoh, H. Y., Hao, Q. Y., Sun, T., Wang, Z. C., Yin, Z. Y., Zhang, Y. P., Lu, J., Bao, Q. L.* & Su, C. L.* High-yield electrochemical production of large-sized and thinly layered NiPS₃ flakes for overall water splitting. Small, 2019, 15, 30, 1902427.

18. Zeb, M. H., Shabbir, B.,* Sagar, R. E., Mahmood, N., Chen, K. Q., Qasim, I., Malik, M. I., Yu, W. Z., Mossain, M., Dai, Z. G., Ou, Q. D., Bhat, M. A., Shivananju, B. N., Li, Y., Tang, X., Qi, K., Younis, A., Khan, Q., Zhang, Y. P.* & Bao, Q. L.* Superior magnetoresistance performance of hybrid graphene foam/metal sulfide nanocrystal devices. ACS Applied Materials and Interface, 2019, 11, 21, 19397-19403.

17. Liu, L. L., Zhang, L., Wang, F., Qi, K., Zhang, H. Y., Cui, X. Q.* & Zheng, W. T.* Bi-metal-organic frameworks type II heterostructures for enhanced photocatalytic styrene oxidation. Nanoscale, 2019, 11, 7554-7559.

16. Ma, X. C., Qi, K., Wei, S. T., Zhang, L.* & Cui, X. Q.* In situ encapsulated nickel-copper nanoparticles in metal-organic frameworks for oxygen evolution reaction. Journal of Alloys and Compounds, 2019, 770, 236-242.

15. Liu. C., Meng, F. L., Zhang, L.,* Zhang, D. T., Wei, S. T., Qi, K., Fan, J. C., Zhang, H. Y. & Cui, X. Q.* CuO/ZnO heterojunction nanoarrays for enhanced photoelectrochemical water oxidation. Applied Surface Science, 2019, 469, 276-282.

2018:

14. Fan, J. C., Yu, S. S., Qi, K., Liu, C., Zhang, L., Zhang, H. Y., Cui, X. Q.* & Zheng, W. T.* Synthesis of ultrathin wrinkle-free PdCu alloy nanosheets for modulating d-band electrons for efficient methanol oxidation. Journal of Materials Chemistry A, 2018, 6, 8531-8536.

13. Zhang, X. L., Cui, X. Q.,* Sun, Y. H., Qi, K., Jin, Z., Wei, S. T., Li, W. W., Zhang, L. J. & Zheng, W. T.* Nanoporous sulfur-doped copper oxide (Cu₂O_xS_1–x) for overall water splitting. ACS Applied Materials and Interfaces, 2018, 10, 1, 745-752.

12. Xu, Y. C., Cui, X. Q.,* Qi, K., Wei. S. T., Wang, Q. Y. & Zheng, W. T.* Interface engineered surface morphology evolution of Au@Pd core-shell nanorods. Nanoscale, 2018, 10, 21161-21167.

2017:

11. Fan, J. C., Qi, K., Zhang, L., Zhang, H. Y., Yu, S. S.* & Cui, X. Q.* Engineering Pt/Pd interfacial electronic structures for highly efficient hydrogen evolution and alcohol oxidation. ACS Applied Materials and Interfaces, 2017, 9, 21, 18008-18014.

10. Fan, J. C., Qi, K., Chen, H., Zheng, W. T. & Cui, X. Q.* Morphology dependence of electrochemical properties on palladium nanocrystals. Journal of Colloid and Interface Science, 2017, 490, 190-196.

9. Zhang, D. T., Liu, L. L. Zhang, L., Qi, K., Zhang, H. Y. & Cui, X. Q.* An anti-photocorrosive photoanode based on a CdS/Ni_xS_y@NF heterostructure for visible-light-driven water splitting. Applied Surface Science, 2017, 420, 161-166.

8. Jin, Z., Liu, C., Qi, K. & Cui, X. Q.* Photo-reduced Cu/CuO nanoclusters on TiO₂ nanotube arrays as highly efficient and reusable catalyst. Scientific Reports, 2017, 7, 39695.

7. Gao, X. D., Liu, L. L., Wang, Q. Y., Qi, K., Jin, Z., Zheng, W. T.* & Cui, X. Q.* One-pot synthesis of nanodendritic PtIr alloy with high electrochemical activity for ethylene glycol oxidation. Nano, 2017, 12, 1750026.

2016:

6. Qi, K., Yu, S. S., Wang, Q. Y., Zhang, W., Fan, J. C., Zheng, W. T.* & Cui. X. Q.* Decoration of the inert basal plane of defect-rich MoS₂ with Pd atoms for achieving Pt-similar HER activity. Journal of Materials Chemistry A, 2016, 4, 4025-4031.

5. Qi, K., Zheng, W. T.* & Cui, X. Q.* Supersaturation-controlled surface structure evolution of Pd@Pt core–shell nanocrystals: enhancement of the ORR activity at a sub-10 nm scale. Nanoscale, 2016, 8, 1698-1703.

4. Wei, S. T., Qi, K., Jin, Z., Cao, J. S., Zheng, W. T., Chen, H. & Cui, X. Q.* One-step synthesis of a self-supported copper phosphide nanobush for overall water splitting. ACS Omega, 2016, 1, 6, 1367-1373.

2015:

3. Wang, Q., Wang, Q. Y., Qi, K., Xue, T. Y., Liu, C., Zheng, W. T.* & Cui, X. Q.* In situ preparation of porous Pd nanotubes on a GCE for non-enzymatic electrochemical glucose sensors. Analytical Methods, 2015, 7, 8605-8610.

2014:

2. Qi, K., Wang, Q. Y., Zheng, W. T.,* Zhang, W. & Cui, X. Q. Porous single-crystalline palladium nanoflowers with enriched {100} facets for highly enhanced ethanol oxidation. Nanoscale, 2014, 6, 15090-15097.

1. Xue, T. Y., Cui, X. Q.,* Guan, W. M., Wang, Q. Y., Liu, C., Wang, H. T., Qi, K., Singh, D. J. & Zheng, W. T.* Surface plasmon resonance technique for directly probing the interaction of DNA and graphene oxide and ultra-sensitive biosensing. Biosensors and Bioelectronics, 2014, 58, 15, 374-379.