高比能锂电池正极材料、固态电池界面问题、电池失效机制

   

080501-材料物理与化学

锂电池，固态电池，电池失效，电池界面问题

2011-09--2014-06   中国科学院物理研究所   博士
2009-09--2011-06   清华大学   联培硕士
2008-09--2011-06   青岛科技大学   硕士
2004-09--2008-06   聊城大学   学士

2018-01~现在, 中国科学院青岛生物能源与过程研究所, 副研究员
2016-08~2017-12,中国科学院青岛生物能源与过程研究所, 助理研究员
2014-07~2016-07,中国科学院青岛生物能源与过程研究所, 博士后

   

[1] 崔光磊, 李文儒, 马君, 徐红霞. 一种分子铁电体晶体包覆的正极材料及其制备方法及其应用. 202210838329.X, 2022-07-18.
[2] 崔光磊, 马君, 孙兴伟, 郑越, 徐红霞, 张舒, 孙德业. 一种高机械强度含包覆层的正极材料、制备方法及其应用. 202210367014.1, 2022-04-08.
[3] 崔光磊, 马君, 王龙龙, 虞鑫润, 姜丰, 孙兴伟, 徐红霞. 一种核壳结构的高电压钴酸锂正极材料及其制备方法. CN: CN109659542B, 2021-08-27.
[4] 崔光磊, 马福瑞, 马君, 韩鹏献, 徐红霞, 张增奇. 一种氟硅烷包覆的复合正极材料及其制备方法和应用. CN: CN112421039A, 2021-02-26.
[5] 崔光磊, 马君, 王龙龙, 孙兴伟, 虞鑫润, 徐红霞. 一种固态锂电池用复合电极材料. 202011101181.9, 2020-10-15.
[6] 崔光磊, 柴敬超, 马君, 徐红霞, 董杉木, 张建军, 鞠江伟, 王鹏. 一种应用于锂电池的宽电位窗口的多级结构复合固态电解质. CN: CN107732297B, 2020-07-14.
[7] 崔光磊, 马君, 虞鑫润, 王龙龙, 徐红霞. 一种选择性浸润聚合物电解质及其制备和应用. CN: CN111342123A, 2020-06-26.
[8] 崔光磊, 张焕瑞, 柴敬超, 王鹏, 马君, 张建军. 耐高电压的固态锂电池聚合物电解质及其制备和应用. CN: CN108242563B, 2020-03-24.
[9] 崔光磊, 马君, 王龙龙, 姜丰, 虞鑫润, 孙兴伟, 徐红霞. 一种高结构稳定性钴酸锂正极材料及其制备方法. CN: CN110336006A, 2019-10-15.
[10] 崔光磊, 马君, 张建军, 张焕瑞, 徐红霞. 一种固态锂电池用低内阻正极材料及其制备方法. CN: CN108232138A, 2018-06-29.
[11] 崔光磊, 马君, 王龙龙, 董杉木, 陈兵兵, 鞠江伟, 徐红霞. 一种玻璃态的氧化物电解质材料. CN: CN107863533A, 2018-03-30.
[12] 崔光磊, 吴天元, 董杉木, 马君, 赵井文, 张建军. 一种基于多物理场的电池健康状态检测与评估方法及装备系统. CN: CN107356879A, 2017-11-17.
[13] 崔光磊, 马君, 刘海胜, 刘兆林, 张欣欣. 一种全固态二次锂电池用改善室温电子离子快速传输电极片的制备方法. CN: CN105932225A, 2016-09-07.
[14] 崔光磊, 赵井文, 董杉木, 马君, 王晓刚. 一种基于锌-磷酸铁锰锂的水系高电压混合离子二次电池. CN: CN105826520A, 2016-08-03.
[15] 马君, 王兆翔, 陈立泉. 二次电池电极材料钼酸锂. CN: CN104577088A, 2015-04-29.

   

[1] Li, Shuwei, Yang, Lu, Liu, Zepeng, Zhang, Chu, Shen, Xi, Gao, Yurui, Kong, Qingyu, Hu, Zhiwei, Kuo, ChangYang, Lin, HongJi, Chen, ChienTe, Yang, Yuan, Ma, Jun, Hu, Zilin, Wang, Xuefeng, Yu, Richeng, Wang, Zhaoxiang, Chen, Liquan. Surface Al-doping for compromise between facilitating oxygen redox and enhancing structural stability of Li-rich layered oxide. ENERGY STORAGE MATERIALS[J]. 2023, 55: 356-363, http://dx.doi.org/10.1016/j.ensm.2022.12.006.
[2] Zhang, Shu, Ma, Jun, Dong, Shanmu, Cui, Guanglei. Designing All-Solid-State Batteries by Theoretical Computation: A Review. ELECTROCHEMICAL ENERGY REVIEWS[J]. 2023, 6(1): 4-, [3] Yantao Wang, Hongtao Qu, Bowen Liu, Xiaoju Li, Jiangwei Ju, Jiedong Li, Shu Zhang, Jun Ma, Chao Li, Zhiwei Hu, Chung-Kai Chang, Hwo-Shuenn Sheu, Longfei Cui, Feng Jiang, Ernst R. H. van Eck, Arno P. M. Kentgens, Guanglei Cui, Liquan Chen. Self-organized hetero-nanodomains actuating super Li + conduction in glass ceramics. NATURE COMMUNICATIONS[J]. 2023, 14(1): 1-11, http://dx.doi.org/10.1038/s41467-023-35982-7.
[4] Zhou, Tong, Yu, Xinrun, Li, Fan, Zhang, Jianwei, Liu, Bowen, Wang, Longlong, Yang, Yuan, Hu, Zhiwei, Ma, Jun, Li, Chao, Cui, Guanglei. Bulk oxygen release inducing cyclic strain domains in Ni-rich ternary cathode materials. ENERGY STORAGE MATERIALS[J]. 2023, 55: 691-697, http://dx.doi.org/10.1016/j.ensm.2022.12.029.
[5] Tiantian Dong, Huanrui Zhang, Lang Huang, Jun Ma, Pengzhou Mu, Xiaofan Du, Xiaohu Zhang, Xiaogang Wang, Chenglong Lu, Shanmu Dong, Qian Zhou, Gaojie Xu, Wei Liu, Guanglei Cui. A smart polymer electrolyte coordinates the trade-off between thermal safety and energy density of lithium batteries. ENERGY STORAGE MATERIALS. 2023, 58: 123-131, http://dx.doi.org/10.1016/j.ensm.2023.03.013.
[6] Yang, Lu, Liu, Zepeng, Shen, Xi, Li, Shuwei, Hu, Zhiwei, Kong, Qingyu, Ma, Jun, Li, Jiedong, Lin, HongJi, Chen, ChienTe, Chen, JinMing, Haw, ShuChih, Wang, Xuefeng, Yu, Richeng, Wang, Zhaoxiang, Chen, Liquan. Effect of vacancy-tailored Mn3+ spinning on enhancing structural stability. ENERGY STORAGE MATERIALS[J]. 2022, 44: 231-238, http://dx.doi.org/10.1016/j.ensm.2021.10.024.
[7] Xingwei Sun, Longlong Wang, Jun Ma, Xinrun Yu, Shu Zhang, Xinhong Zhou, Guanglei Cui. A Bifunctional Chemomechanics Strategy To Suppress Electrochemo-Mechanical Failure of Ni-Rich Cathodes for All-Solid-State Lithium Batteries. Acs Applied Materials & Interfaces[J]. 2022, 14: 17674-17681, [8] Zhang, YuHan, Zhang, Ding, Wu, LinRong, Ma, Jun, Yi, Qun, Wang, Zhaoxiang, Wang, Xuefeng, Wu, Zhen, Zhang, Chu, Hu, Naifang, Haw, ShuChih, Chen, JinMing, Hu, Zhiwei, Cui, Guanglei. Stabilization of Lattice Oxygen in Li-Rich Mn-Based Oxides via Swing-like Non-Isothermal Sintering. ADVANCED ENERGY MATERIALS[J]. 2022, 12(43): http://dx.doi.org/10.1002/aenm.202202341.
[9] Liu, Bowen, Hu, Naifang, Li, Chao, Ma, Jun, Zhang, Jianwei, Yang, Yuan, Sun, Deye, Yin, Bangxun, Cui, Guanglei. Direct Observation of Li-Ion Transport Heterogeneity Induced by Nanoscale Phase Separation in Li-rich Cathodes of Solid-State Batteries. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2022, 61(40): e202209626-, http://dx.doi.org/10.1002/anie.202209626.
[10] Liu, Zepeng, Liu, Shuai, Yang, Lu, Zhang, Chu, Shen, Xi, Zhang, Qinghua, Lin, HongJi, Chen, ChineTe, Hu, Zhiwei, Yang, Yuan, Ma, Jun, Yu, Richeng, Wang, Xuefeng, Wang, Zhaoxiang, Chen, Liquan. Feasibility to Improve the Stability of Lithium-Rich Layered Oxides by Surface Doping. ACS APPLIED MATERIALS & INTERFACES[J]. 2022, 14(16): 18353-18359, http://dx.doi.org/10.1021/acsami.2c00155.
[11] Du, Xiaofan, Lu, Guoli, Shao, Zhipeng, Wang, Chengdong, Ma, Jun, Zhao, Jingwen, Cui, Guanglei. Theoretical insight into lithium triborates as solid-state electrolytes. APPLIED PHYSICS LETTERS[J]. 2022, 121(24): [12] Sun, Jinran, Zhang, Shu, Zhang, Qinghua, Xin, Yunchuan, Dong, Shamu, Liu, Haisheng, Li, Jiedong, Wang, Chao, Lu, Chenglong, Yang, Wuhai, Liu, Tingting, Ma, Jun, Gu, Lin, Cui, Guanglei. Unshackling the reversible capacity of SiOx/graphite-based full cells via selective LiF-induced lithiation. SCIENCE CHINA-MATERIALS[J]. 2022, 65(9): 2335-2342, http://dx.doi.org/10.1007/s40843-021-2049-9.
[13] Li, Shuwei, Liu, Zepeng, Yang, Lu, Shen, Xi, Liu, Qiuyan, Hu, Zhiwei, Kong, Qingyu, Ma, Jun, Li, Jiedong, Lin, HongJi, Chen, ChienTe, Wang, Xuefeng, Yu, Richeng, Wang, Zhaoxiang, Chen, Liquan. Anionic redox reaction and structural evolution of Ni-rich layered oxide cathode material. NANO ENERGY[J]. 2022, 98: http://dx.doi.org/10.1016/j.nanoen.2022.107335.
[14] 虞鑫润, 马君, 牟春博, 崔光磊. 高锂离子电导的有机-无机复合电解质的渗流结构设计. 物理化学学报[J]. 2022, 38(3): 1912061-, [15] Li, Longshan, Wang, Dingming, Xu, Gaojie, Zhou, Qian, Ma, Jun, Zhang, Jianjun, Du, Aobing, Cui, Zili, Zhou, Xinhong, Cui, Guanglei. Recent progress on electrolyte functional additives for protection of nickel-rich layered oxide cathode materials. JOURNAL OF ENERGY CHEMISTRY[J]. 2022, 65(2): 280-292, http://dx.doi.org/10.1016/j.jechem.2021.05.049.
[16] Wang, Longlong, Sun, Xingwei, Ma, Jun, Chen, Bingbing, Li, Chao, Li, Jiedong, Chang, Liang, Yu, Xinrun, Chan, TingShan, Hu, Zhiwei, Noked, Malachi, Cui, Guanglei. Bidirectionally Compatible Buffering Layer Enables Highly Stable and Conductive Interface for 4.5 V Sulfide-Based All-Solid-State Lithium Batteries. ADVANCED ENERGY MATERIALS[J]. 2021, 11(32): 2100881-, http://dx.doi.org/10.1002/aenm.202100881.
[17] Wang, Xiao, Sun, Jujie, Feng, Changhao, Wang, Xiujuan, Xu, Minghan, Sun, Jingjiang, Zhang, Ning, Ma, Jun, Wang, Qingfu, Zong, Chengzhong, Cui, Guanglei. Lithium bis(oxalate)borate crosslinked polymer electrolytes for high-performance lithium batteries. JOURNAL OF ENERGY CHEMISTRY[J]. 2021, 55(4): 228-235, http://dx.doi.org/10.1016/j.jechem.2020.06.070.
[18] Ma, Yue, Wang, Chengdong, Ma, Jun, Xu, Gaojie, Chen, Zheng, Du, Xiaofan, Zhang, Shu, Zhou, Xinhong, Cui, Guanglei, Chen, Liquan. Interfacial chemistry of gamma-glutamic acid derived block polymer binder directing the interfacial compatibility of high voltage LiNi0.5Mn1.5O4 electrode. SCIENCE CHINA-CHEMISTRY[J]. 2021, 64(1): 92-100, http://dx.doi.org/10.1007/s11426-020-9879-8.
[19] Chen, Hao, Adekoya, David, Hencz, Luke, Ma, Jun, Chen, Su, Yan, Cheng, Zhao, Huijun, Cui, Guanglei, Zhang, Shanqing. Stable Seamless Interfaces and Rapid Ionic Conductivity of Ca-CeO2/LiTFSI/PEO Composite Electrolyte for High-Rate and High-Voltage All-Solid-State Battery. ADVANCED ENERGY MATERIALS[J]. 2020, 10(21): https://www.webofscience.com/wos/woscc/full-record/WOS:000539283600005.
[20] Wu, Han, Tang, Ben, Du, Xiaofan, Zhang, Jianjun, Yu, Xinrun, Wang, Yantao, Ma, Jun, Zhou, Qian, Zhao, Jingwen, Dong, Shanmu, Xu, Gaojie, Zhang, Jinning, Xu, Hai, Cui, Guanglei, Chen, Liquan. LiDFOB Initiated In Situ Polymerization of Novel Eutectic Solution Enables Room-Temperature Solid Lithium Metal Batteries. ADVANCED SCIENCE[J]. 2020, 7(23): http://apps.webofknowledge.com/CitedFullRecord.do?product=UA&colName=WOS&SID=5CCFccWmJJRAuMzNPjj&search_mode=CitedFullRecord&isickref=WOS:000584473600001.
[21] Lu, Tao, Zhang, Zhonghua, Chen, Bingbing, Dong, Shanmu, Wang, Chengdong, Du, Aobing, Wang, Longlong, Ma, Jun, Cui, Guanglei. A superior electronic conducting tellurium electrode enabled high rate capability rechargeable Mg batteries. MATERIALS TODAY ENERGY[J]. 2020, 17: http://dx.doi.org/10.1016/j.mtener.2020.100450.
[22] Cheng, Xiangyang, Zhang, Zhonghua, Kong, Qingyu, Zhang, Qinghua, Wang, Tao, Dong, Shanmu, Gu, Lin, Wang, Xiao, Ma, Jun, Han, Pengxian, Lin, Hongji, Chen, ChienTe, Cui, Guanglei. Highly Reversible Cuprous Mediated Cathode Chemistry for Magnesium Batteries. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION[J]. 2020, 59(28): 11477-11482, http://dx.doi.org/10.1002/anie.202002177.
[23] Hu, Rongxiang, Qiu, Huayu, Zhang, Huanrui, Wang, Peng, Du, Xiaofan, Ma, Jun, Wu, Tianyuan, Lu, Chenglong, Zhou, Xinhong, Cui, Guanglei. A Polymer-Reinforced SEI Layer Induced by a Cyclic Carbonate-Based Polymer Electrolyte Boosting 4.45 V LiCoO2/Li Metal Batteries. SMALL[J]. 2020, 16(13): http://dx.doi.org/10.1002/smll.201907163.
[24] Yu, Xinrun, Wang, Longlong, Ma, Jun, Sun, Xingwei, Zhou, Xinhong, Cui, Guanglei. Selectively Wetted Rigid-Flexible Coupling Polymer Electrolyte Enabling Superior Stability and Compatibility of High-Voltage Lithium Metal Batteries. ADVANCED ENERGY MATERIALS[J]. 2020, 10(18): https://www.webofscience.com/wos/woscc/full-record/WOS:000520736400001.
[25] Xu, Gaojie, Han, Pengxian, Wang, Xiao, Zhou, Xinhong, Han, Xiaoqi, Lu, Di, Liu, Haisheng, Zhao, Jingwen, Ma, Jun, Cui, Guanglei. A High-Energy 5 V-Class Flexible Lithium-Ion Battery Endowed by Laser-Drilled Flexible Integrated Graphite Film. ACS APPLIED MATERIALS & INTERFACES[J]. 2020, 12(8): 9468-9477, https://www.webofscience.com/wos/woscc/full-record/WOS:000517360000053.
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[27] Longlong Wang, Ruicong Xie, Bingbing Chen, Xinrun Yu, Jun Ma, Chao Li, Zhiwei Hu, Xingwei Sun, Chengjun Xu, Shanmu Dong, TingShan Chan, Jun Luo, Guanglei Cui, Liquan Chen. In-situ visualization of the space-charge-layer effect on interfacial lithium-ion transport in all-solid-state batteries. NATURE COMMUNICATIONS[J]. 2020, 11(1): https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7674427/.
[28] Ju, Jiangwei, Ma, Jun, Wang, Yantao, Cui, Yanyan, Han, Pengxian, Cui, Guanglei. Solid-state energy storage devices based on two-dimensional nano-materials. ENERGY STORAGE MATERIALSnull. 2019, 20: 269-290, http://dx.doi.org/10.1016/j.ensm.2018.11.025.
[29] Ma, Yue, Chen, Kai, Ma, Jun, Xu, Gaojie, Dong, Shanmu, Chen, Bingbing, Li, Jiedong, Chen, Zheng, Zhou, Xinhong, Cui, Guanglei. A biomass based free radical scavenger binder endowing a compatible cathode interface for 5 V lithium-ion batteries. ENERGY & ENVIRONMENTAL SCIENCE[J]. 2019, 12(1): 273-280, https://www.webofscience.com/wos/woscc/full-record/WOS:000457194500017.
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[32] Zhou, Qian, Ma, Jun, Dong, Shanmu, Li, Xianfeng, Cui, Guanglei. Intermolecular Chemistry in Solid Polymer Electrolytes for High-Energy-Density Lithium Batteries. ADVANCED MATERIALS[J]. 2019, 31(50): https://www.webofscience.com/wos/woscc/full-record/WOS:000483161700001.
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[35] Zhang, Xinxin, Ma, Jun, Hu, Pu, Chen, Bingbing, Lu, Chenglong, Zhou, Xinhong, Han, Pengxian, Chen, Lihua, Cui, Guanglei. An insight into failure mechanism of NASICON-structured Na3V2(PO4)(3) in hybrid aqueous rechargeable battery. JOURNAL OF ENERGY CHEMISTRY[J]. 2019, 32(5): 1-7, http://lib.cqvip.com/Qikan/Article/Detail?id=7002016268.
[36] Xu, Hantao, Zhang, Huanrui, Ma, Jun, Xu, Gaojie, Dong, Tiantian, Chen, Jinchun, Cui, Guanglei. Overcoming the Challenges of 5 V Spinel LiNi0.5Mn1.5O4 Cathodes with Solid Polymer Electrolytes. ACS ENERGY LETTERSnull. 2019, 4(12): 2871-2886, https://www.webofscience.com/wos/woscc/full-record/WOS:000503114500014.
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[40] Zhang, Shu, Ma, Jun, Hu, Zhenglin, Cui, Guanglei, Chen, Liquan. Identifying and Addressing Critical Challenges of High-Voltage Layered Ternary Oxide Cathode Materials. CHEMISTRY OF MATERIALSnull. 2019, 31(16): 6033-6065, https://www.webofscience.com/wos/woscc/full-record/WOS:000483435400002.
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[46] Du, Huiping, Li, Shizhen, Qu, Hongtao, Lu, Boyang, Wang, Xiaogang, Chai, Jingchao, Zhang, Huanrui, Ma, Jun, Zhang, Zhonghua, Cui, Guanglei. Stable cycling of lithium-sulfur battery enabled by a reliable gel polymer electrolyte rich in ester groups. JOURNAL OF MEMBRANE SCIENCE[J]. 2018, 550: 399-406, http://dx.doi.org/10.1016/j.memsci.2018.01.017.
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（ 1 ） 全固态聚合物锂电池的性能衰减机理和改性研究, 主持, 省级, 2017-05--2019-12
（ 2 ） 高电压钴酸锂电池聚合物电解质研究, 主持, 省级, 2016-07--2019-12
（ 3 ） 基于含金属-金属键层状结构正极材料的高比能、长寿命型锂离子电池研究, 主持, 省级, 2015-07--2017-07
（ 4 ） 前、后过渡金属在高电压层状结构正极材料中的协同作用机制, 主持, 国家级, 2016-01--2018-12
（ 5 ） 高比能固态聚合物锂电池界面失效机理研究及提升策略, 主持, 国家级, 2020-01--2023-12
（ 6 ） 高能量密度长循环寿命硫化物基固态锂电池的界面设计与构筑, 主持, 省级, 2021-01--2023-12
（ 7 ） 固态锂电池, 主持, 部委级, 2021-01--2024-12
（ 8 ） 无机固态锂电池电-化-力多场耦合效应对载流子 输运特性的影响与调控, 主持, 市地级, 2021-06--2023-05

（1）钴酸锂/硫化物电解质界面锂传输的原位可视化研究   第十届纳米与新能源技术青年科学家论坛   2020-10-10
（2）共改性策略改善高电压钴酸锂的结构和界面稳定性   第四届青岛储能技术论坛暨第一届多价金属离子   2019-05-11

与中国科学院物理研究所、天津理工大学、青岛科技大学、青岛大学、南京工业大学、法国SOLEIL同步辐射光源、德国马普固体化学物理研究所等建立了稳定的合作关系。