新型金属氢化物储氢及其功能化研究

080501-材料物理与化学

储氢材料，储氢系统，催化，电化学

2011-09--2014-09   大连理工大学-大连化学物理研究所联培   博士
2008-09--2011-06   湘潭大学   硕士
2004-09--2008-06   湘潭大学   学士

   

2018-12~现在, 中国科学院大连化学物理研究所, 副研究员
2014-12~2018-11,德国Helmholtz-Zentrum Geesthacht, 博士后

2020-12-01-2025-09-29,全国氢能标准化技术委员会委员, 委员

   

（1） 壳牌氢能关键技术挑战赛, 其他, 2019
（2） 延长石油奖学金, 二等奖, 研究所（学校）, 2014
（3） 大连市青年文明号, 市地级, 2014

（ 1 ） 一种TiO2基催化剂、其制备方法及应用, 发明专利, 2023, 第 1 作者, 专利号: CN116493030A

（ 2 ） 一种催化剂及其制备方法和含有该催化剂的储氢材料及其制备方法, 发明专利, 2023, 第 1 作者, 专利号: CN115957734A

（ 3 ） 一种金属氮基储氢材料在氢同位素分离中的应用和金属氮化物的制备方法, 发明专利, 2022, 第 1 作者, 专利号: CN114618300A

（ 4 ） 一种含钛物质催化改性镁基储氢材料及其制备方法与应用, 发明专利, 2022, 第 1 作者, 专利号: CN114620676A

（ 5 ） 一种多元金属含氢化合物的制备方法, 发明专利, 2021, 第 3 作者, 专利号: CN112978679A

（ 6 ） 一种聚合物包覆储氢材料及其制备方法和应用, 发明专利, 2021, 第 1 作者, 专利号: CN112390224A

（ 7 ） 一种制备储氢材料的方法, 发明专利, 2021, 第 1 作者, 专利号: CN112299366A

（ 8 ） 一种廉价大规模制备氮基金属化合物储氢材料的方法, 专利授权, 2016, 第 2 作者, 专利号: CN105776132A

（ 9 ） 金属氮基化合物储氢材料热力学性能的改善方法, 发明专利, 2015, 第 2 作者, 专利号: CN104649223A

   

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[2] 陈佳琪, 高文波, 朱良柱, 陶浩良, 冯圣, 曹湖军, 郭建平, 陈艳霞, 陈萍. A mixed proton–electron-conducting cathode with a Ru nanoparticle catalyst for electrochemical ammonia synthesis based on a proton-conducting BZCYYb electrolyte. Journal of Materials Chemistry A[J]. 2024, 第 6 作者null(null): https://pubs.rsc.org/en/content/articlehtml/2024/ta/d4ta04520c.
[3] Bolarin, Joshua Adedeji, Zou, Ren, Li, Zhi, Munyentwali, Alexis, Zhang, Zhao, Cao, Hujun. Recent path to ultrafine Mg/MgH2 synthesis for sustainable hydrogen storage. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY[J]. 2024, 第 6 作者  通讯作者  52: 251-274, http://dx.doi.org/10.1016/j.ijhydene.2023.04.234.
[4] 关业勤, 文红, 崔开勋, 王倩茹, 高文波, 蔡永丽, 程咨博, 裴启俊, 李曌, 曹湖军, 何腾, 郭建平, 陈萍. Light-driven ammonia synthesis under mild conditions using lithium hydride. Nature Chemistry[J]. 2024, 第 10 作者16: 373-379, 
[5] Zou, Ren, Zhang, Weijin, Dai, Min, Lei, Gangtie, Jiang, Qike, Cao, Hujun, Chen, Ping. One-Step Synthesis of Light Metal Nanoparticle from Metastable Complex. SMALL[J]. 2023, 第 6 作者  通讯作者  19(8): http://dx.doi.org/10.1002/smll.202206518.
[6] 张炜进, 崔继荣, 王上上, 曹湖军, 吴安安, 夏元华, 蒋齐可, 郭建平, 何腾, 陈萍. Deforming lanthanum trihydride for superionic conduction. Nature[J]. 2023, 第 4 作者  通讯作者  616(7955): 73-76, https://doi.org/10.1038/s41586-023-05815-0.
[7] Zou, Ren, Li, Jialing, Cui, Jirong, Zhang, Weijin, Lei, Gangtie, Cao, Hujun, Chen, Ping. Catalyst-free synthesis of lithium hydride at room temperature. CHEMICAL COMMUNICATIONS[J]. 2023, 第 6 作者  通讯作者  59(18): 2660-2663, http://dx.doi.org/10.1039/d2cc06849d.
[8] Feng, Sheng, Gao, Wenbo, Guo, Jianping, Cao, Hujun, Chen, Ping. Electrodriven Chemical Looping Ammonia Synthesis Mediated by Lithium Imide. ACS Energy Letters[J]. 2023, 第 4 作者  通讯作者  8(3): 1567-1574, 
[9] Han Wu, Liang Yang, Jiaqi Wen, Yongfeng Xu, Yongli Cai, Wenbo Gao, Qianru Wang, Yeqin Guan, Sheng Feng, Hujun Cao, Teng He, Lin Liu, Shaoqian Zhang, Jianping Guo, Ping Chen. Plasma-Driven Nitrogen Fixation on Sodium Hydride. Advanced Energy Materials[J]. 2023, 第 10 作者2300722: 
[10] 程咨博, 邹韧, 曹湖军. 外场在轻金属氢化物储氢体系中的应用. 中国材料进展[J]. 2023, 第 3 作者42(1): 10-19, http://lib.cqvip.com/Qikan/Article/Detail?id=7109180917.
[11] Cao, Hujun, Pistidda, Claudio, Richter, Theresia M M, Capurso, Giovanni, Milanese, Chiara, Tseng, JoChi, Shang, Yuanyuan, Niewa, Rainer, Chen, Ping, Klassen, Thomas, Dornheim, Martin. De-hydrogenation/Rehydrogenation Properties and Reaction Mechanism of A(m)Zn(NH2)(n)-2nLiH Systems (A = Li, K, Na, and Rb). SUSTAINABILITY[J]. 2022, 第 1 作者14(3): http://dx.doi.org/10.3390/su14031672.
[12] 王江, 雷刚铁, 何腾, 曹湖军, 陈萍. Defect-rich potassium amide: A new solid-state potassium ion electrolyte. Journal of Energy Chemistry[J]. 2022, 第 4 作者  通讯作者  69: 555-560, 
[13] Min Dai, Joshua Adedeji Bolarin, Gangtie Lei, Zhi Li, Teng He, Hujun Cao, Ping Chen. Potassium hydride reduced black TiO2−x for boosting the hydrogenation of magnesium at room temperature. JOURNAL OF ALLOYS AND COMPOUNDS[J]. 2022, 第 6 作者  通讯作者  897: 
[14] Zou, Ren, Bolarin, Joshua Adedeji, Lei, Gangtie, Gao, Wenbo, Li, Zhi, Cao, Hujun, Chen, Ping. Microwave-assisted reduction of Ti species in MgH2-TiO2 composite and its effect on hydrogen storage. Chemical Engineering Journal[J]. 2022, 第 6 作者  通讯作者  450: 138072, 
[15] Yuan, Zirui, Li, Shaohan, Wang, Kaiwen, Xu, Nuo, Sun, Weiwei, Sun, Litao, Cao, Hujun, Lin, Huaijun, Zhu, Yunfeng, Zhang, Yao. in-situ formed Pt nano-clusters serving as destabilization-catalysis bi-functional additive for MgH2. CHEMICAL ENGINEERING JOURNAL[J]. 2022, 第 7 作者435: http://dx.doi.org/10.1016/j.cej.2022.135050.
[16] Dai Min, Lei Gangtie, Zhang Zhao, Li Zhi, Cao Hujun, Chen Ping. Room Temperature Hydrogen Absorption of V2O5 Catalyzed MgH2/Mg. ACTA CHIMICA SINICA[J]. 2022, 第 5 作者  通讯作者  80(3): 303-309, http://dx.doi.org/10.6023/A21120561.
[17] Bolarin, Joshua Adedeji, Zou, Ren, Li, Zhi, Zhang, Zhao, Cao, Hujun. MXenes for magnesium-based hydrides: A review. APPLIED MATERIALS TODAY. 2022, 第 5 作者  通讯作者  29: http://dx.doi.org/10.1016/j.apmt.2022.101570.
[18] Yan, Hanxue, Gao, Wenbo, Cui, Jirong, Zhang, Weijin, Pei, Qijun, Wang, Qianru, Guan, Yeqin, Feng, Sheng, Wu, Han, Cao, Hujun, Guo, Jianping, Chen, Ping. Dinitrogen fixation mediated by lanthanum hydride. Journal of Energy Chemistry[J]. 2022, 第 10 作者72(9): 1-7, 
[19] Pei, Qijun, He, Teng, Yu, Yang, Jing, Zijun, Wang, Jintao, Tan, Khai Chen, Guo, Jianping, Liu, Lin, Cao, Hujun, Chen, Ping. Fabrication of oxygen vacancies through assembling an amorphous titanate overlayer on titanium oxide for a catalytic water-gas shift reaction. JOURNAL OF MATERIALS CHEMISTRY A[J]. 2021, 第 9 作者9(5): 2784-2791, http://dx.doi.org/10.1039/d0ta11641f.
[20] Wang, Qianru, Pan, Jaysree, Guo, Jianping, Hansen, Heine Anton, Xie, Hua, Jiang, Ling, Hua, Lei, Li, Haiyang, Guan, Yeqin, Wang, Peikun, Gao, Wenbo, Liu, Lin, Cao, Hujun, Xiong, Zhitao, Vegge, Tejs, Chen, Ping. Ternary ruthenium complex hydrides for ammonia synthesis via the associative mechanism. Nature Catalysis[J]. 2021, 第 13 作者4(11): 959, 
[21] Bolarin, Joshua Adedeji, Zhang, Zhao, Cao, Hujun, Li, Zhi, He, Teng, Chen, Ping. Room Temperature Hydrogen Absorption of Mg/MgH2 Catalyzed by BaTiO3. JOURNAL OF PHYSICAL CHEMISTRY C[J]. 2021, 第 3 作者  通讯作者  125(36): 19631-19641, http://dx.doi.org/10.1021/acs.jpcc.1c05560.
[22] He, Teng, Cao, Hujun, Chen, Ping. The Roles of Alkali/Alkaline Earth Metals in the Materials Design and Development for Hydrogen Storage. ACCOUNTS OF MATERIALS RESEARCH[J]. 2021, 第 2 作者2(9): 726-738, 
[23] Wang, Jiang, Lei, Gangtie, Pistidda, Claudio, He, Teng, Cao, Hujun, Dornheim, Martin, Chen, Ping. Hydrogen storage properties and reaction mechanisms of K2Mn(NH2)(4)-8LiH system. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY[J]. 2021, 第 5 作者  通讯作者  46(80): 40196-40202, http://dx.doi.org/10.1016/j.ijhydene.2021.09.216.
[24] Feng, Sheng, Gao, Wenbo, Wang, Qianru, Guan, Yeqin, Yan, Hanxue, Wu, Han, Cao, Hujun, Guo, Jianping, Chen, Ping. A multi-functional composite nitrogen carrier for ammonia production via a chemical looping route. Journal of Materials Chemistry A[J]. 2021, 第 7 作者  通讯作者  9(2): 1039-1047, 
[25] Zhang, Zhao, Cao, Hujun, Xiong, Zhitao, Bolarin, Joshua Adedeji, Zhang, Weijin, Chen, Ping. Can nitrogen-based complex hydrides be a hydrogen isotope separation material?. CHEMICAL COMMUNICATIONS[J]. 2021, 第 2 作者  通讯作者  57(78): 10063-10066, http://dx.doi.org/10.1039/d1cc03825g.
[26] Yan, Hanxue, Gao, Wenbo, Wang, Qianru, Guan, Yeqin, Feng, Sheng, Wu, Han, Guo, Qing, Cao, Hujun, Guo, Jianping, Chen, Ping. Lithium Palladium Hydride Promotes Chemical Looping Ammonia Synthesis Mediated by Lithium Imide and Hydride. The Journal of Physical Chemistry C[J]. 2021, 第 8 作者125(12): 6716-6722, 
[27] Joshua AdedejiBolarin, 张钊, 曹湖军, 李智, 何腾, 陈萍. NaH doped TiO2 as a high-performance catalyst for Mg/MgH2 cycling stability and room temperature absorption. Journal of Magnesium and Alloys[J]. 2021, 第 3 作者  通讯作者  
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[29] Cao, Hujun, Pistidda, Claudio, Castro Riglos, Maria Victoria, Chaudhary, AnnaLisa, Capurso, Giovanni, Tseng, JoChi, Puszkiel, Julian, Wharmby, Michael T, Gemming, Thomas, Chen, Ping, Klassen, Thomas, Dornheim, Martin. Conversion of magnesium waste into a complex magnesium hydride system: Mg(NH2)(2)-LiH. SUSTAINABLE ENERGY & FUELS[J]. 2020, 第 1 作者  通讯作者  4(4): 1915-1923, https://www.webofscience.com/wos/woscc/full-record/WOS:000526855200035.
[30] Zhang, Zhao, Cao, Hujun, Zhang, Weijin, Cui, Jirong, Xiong, Zhitao, Chen, Ping. Thermochemical transformation and reversible performance of Mg(NH2)(2)-NaMgH3 system. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY[J]. 2020, 第 2 作者  通讯作者  45(43): 23069-23075, http://dx.doi.org/10.1016/j.ijhydene.2020.06.094.
[31] Jirong Cui, Weijin Zhang, Hujun Cao, Ping Chen. Mild-condition synthesis of A2ZnH4 (A = K, Rb, Cs) and their effects on the hydrogen storage properties of 2LiH-Mg(NH2)2. Journal of Energy Chemistry[J]. 2020, 第 3 作者  通讯作者  50: 358-364, https://www.sciengine.com/doi/10.1016/j.jechem.2020.03.067.
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[41] Wang, Han, Cao, Hujun, Wu, Guotao, He, Teng, Chen, Ping. The improved Hydrogen Storage Performances of the Multi-Component Composite: 2Mg(NH2)(2)-3LiH-LiBH4. ENERGIES[J]. 2015, 第 2 作者8(7): 6898-6909, http://cas-ir.dicp.ac.cn/handle/321008/146478.
[42] Cao, Hujun, Richter, Theresia M M, Pistidda, Claudio, Chaudhary, AnnaLisa, Santoru, Antonio, Gizer, Goekhan, Niewa, Rainer, Chen, Ping, Klassen, Thomas, Dornheim, Martin. Ternary Amides Containing Transition Metals for Hydrogen Storage: A Case Study with Alkali Metal Amidozincates. CHEMSUSCHEM[J]. 2015, 第 1 作者  通讯作者  8(22): 3777-3782, http://cas-ir.dicp.ac.cn/handle/321008/171580.
[43] Hujun Cao, Theresia M M Richter, Claudio Pistidda, AnnaLisa Chaudhary, Antonio Santoru, Gouml, khan Gizer, Rainer Niewa, 陈萍, Thomas Klassen and Martin Dornheim. Ternary Amides Containing Transition Metals for Hydrogen Storge: A Case Study with Alkali Metal Amidozincates. CHEMSUSCHEM[J]. 2015, 第 1 作者8: 3777, http://cas-ir.dicp.ac.cn/handle/321008/148228.
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[45] Cao, Hujun, Wang, Han, He, Teng, Wu, Guotao, Xiong, Zhitao, Qiu, Jieshan, Chen, Ping. Improved kinetics of the Mg(NH2)(2)-2LiH system by addition of lithium halides. RSC ADVANCES[J]. 2014, 第 1 作者4(61): 32555-32561, http://cas-ir.dicp.ac.cn/handle/321008/144283.
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[51] 曹湖军, Yao Zhang, 王涵, 何腾, 熊智涛, 吴国涛, 陈萍. Modified Hydrogen Storage Performance of Mg(NH2)2/LiH Composite. europea hydrogen energy conference 2014. 2014, 第 1 作者23, http://159.226.238.44/handle/321008/120004.
[52] 陈萍, 陈君儿, 曹湖军, 吴国涛, 熊智涛. Nitrogen based materials for hydrogen storage. 14th international symposium on metal-hydrogen systems. 2014, 第 3 作者169, http://159.226.238.44/handle/321008/119945.
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（1） 氢化物：载氢载能体, 科学出版社, 2021-06, 第 4 作者

   

（ 1 ） 钾(铷)基三元过渡金属氢化物对氨基镁-氢化锂体系储氢性能的影响及其作用机理的研究, 主持, 国家级, 2019-01--2021-12
（ 2 ） 高密度储氢体系的开发、规模化制备及系统集成 技术, 主持, 省级, 2021-01--2023-12
（ 3 ） 高密度储氢材料及其可逆吸/放氢技术, 主持, 国家级, 2021-12--2025-11
（ 4 ） 中国科学院青年创新促进会, 主持, 部委级, 2019-01--2022-12

Martin Dornheim教授, Helmholtz-Zentrum Geesthacht, Germany

Hui Wu教授, NIST, USA

Chiara Milanese教授, University of Pavia, Italy

Rainer Niewa教授, University of Stuttgart, Germany

现指导学生

程咨博  硕士研究生  085600-材料与化工