催化材料制备、表征、反应机理研究

颗粒在流体中的成像研究

物理学、光学、化工流体力学

081701-化学工程
080501-材料物理与化学
070304-物理化学

颗粒在流体中的成像
能源技术产业链耦合技术研究
分子筛材料在催化甲醇转化反应中的机理研究

2004-07--2009-08   中国科学院大连化学物理研究所   理学博士
2003-08--2004-07   中国科学技术大学   代培
1997-09--2001-07   太原理工大学   学士

博士研究生毕业

理学博士

   

2015-03~2016-04,美国加利福尼亚大学洛杉矶分校, 联培访问学者
2013-07~现在, 中国科学院大连化学物理研究所, 副研究员
2009-10~2013-07,中国科学院大连化学物理研究所, 助理研究员
2003-04~2003-08,中国科学院大连化学物理研究所, 研究实习员
2001-07~2003-04,山西海泰克化工新技术有限公司, 研发助理

2020-09-01-2023-09-01,沈阳化工大学硕士研究生校外导师,

   

[1] 叶茂, 马丽坤, 丁亚, 徐庶亮, 刘中民. 流体力学可视化测量的多孔材料及其制备方法和应用. CN: CN111256944B, 2021-05-25.

[2] 杨维慎, 王丽霞, 徐庶亮, 楚文玲, 丛铀. 一种乙烯气相直接氧化制乙酸催化剂及其制备方法. CN: CN101811045A, 2010-08-25.

[3] 杨维慎, 徐庶亮, 王丽霞, 楚文玲, 丛铀. 一种乙烯气相直接氧化制乙酸催化材料的制备方法. CN: CN101780410A, 2010-07-21.

[4] 叶茂, 张涛, 张今令, 徐庶亮, 唐海龙, 王贤高, 张骋, 贾金明, 王静, 李华, 李承功, 刘中民. 流化床反应器、装置以及含氧化合物制备低碳烯烃的方法. CN: CN114377620A, 2022-04-22.

[5] 张涛, 叶茂, 张今令, 徐庶亮, 唐海龙, 王贤高, 张骋, 贾金明, 王静, 李华, 李承功, 刘中民. 一种焦调控反应器、由含氧化合物制备低碳烯烃的装置和应用. CN: CN114377624A, 2022-04-22.

[6] 叶茂, 张涛, 张今令, 徐庶亮, 唐海龙, 王贤高, 张骋, 贾金明, 王静, 李华, 李承功, 刘中民. 一种流化床反应器、装置以及应用. CN: CN114377621A, 2022-04-22.

[7] 张涛, 叶茂, 张今令, 徐庶亮, 唐海龙, 王贤高, 张骋, 贾金明, 王静, 李华, 李承功, 刘中民. 焦调控反应器、装置及含氧化合物制备低碳烯烃的方法. CN: CN114377625A, 2022-04-22.

[8] 叶茂, 张涛, 张今令, 徐庶亮, 唐海龙, 王贤高, 张骋, 贾金明, 王静, 李华, 李承功, 刘中民. 流化床再生器、制备低碳烯烃的装置及其应用. CN: CN114377729A, 2022-04-22.

[9] 张涛, 叶茂, 张今令, 徐庶亮, 唐海龙, 王贤高, 张骋, 贾金明, 王静, 李华, 李承功, 刘中民. 再生装置、制备低碳烯烃的装置及其应用. CN: CN114377730A, 2022-04-22.

1.  Ma Likun, Guo Qiang, Li Xue, Xu Shuliang, Zhou Jibin, Ye Mao, Liu Zhongmin. Drag correlations for flow past monodisperse arrays of spheres and porous spheres based on symbolic regression: Effects of permeability. Chemical Engineering Journal, 2022, DOI: 10.1016/j.cej.2022.136653.

2.  Ma Likun, Kashanj Sina, Xu Shuliang, Zhou Jibin, Nobes David, Ye Mao. Flow reconstruction and prediction based on small particle image velocimetry experimental datasets with convolutional neural networks. Industrial & Engineering Chemistry Research, 2022, DOI: 10.1021/acs.iecr.1c04704.

3.  Guo Qiang, Bordbar Alireza, Ma Likun, Yu Yaxiong, Xu Shuliang, Boyce Christopher M., Ye Mao. A CFD-DEM study of the solid-like and fluid-like states in the homogeneous fluidization regime of Geldart A particles. AIChE Journal, 2022, 68: e17420, DOI: 10.1002/aic.17420.

4.  梁金强, 刘丹竹, 徐庶亮, 叶茂, 刘中民. “双碳”目标下能源安全定量评价方法. 化工进展, 2022, 41: 1622-1633, DOI: 10.16085/j.issn.1000-6613.2021-2255.

5.  Niu Yiming, Huang Xing, Wang Yongzhao, Xu Ming, Chen Junnan, Xu Shuliang, Willinger Marc-Georg, Zhang Wei, Wei Min, Zhang Bingsen. Manipulating interstitial carbon atoms in the nickel octahedral site for highly efficient hydrogenation of alkyne. NATURE COMMUNICATIONS, 2020, 11 (1), DOI: 10.1038/s41467-020-17188-3.

[1] Liu, Danzhu, Liang, Jinqiang, Xu, Shuliang, Ye, Mao. Analysis of Carbon Emissions Embodied in the Provincial Trade of China Based on an Input-Output Model and k-Means Algorithm. Sustainability[J]. 2023, 第 3 作者15(12): http://dx.doi.org/10.3390/su15129196.
[2] Liang, Jinqiang, Liu, Danzhu, Xu, Shuliang, Ye, Mao. Comparison of light olefins production routes in China: Combining techno-economics and security analysis. Chemical Engineering Research and Design[J]. 2023, 第 3 作者  通讯作者  194: 225-241, http://dx.doi.org/10.1016/j.cherd.2023.04.037.
[3] Likun Ma, Sina Kashanj, Xue Li, Shuliang Xu, David S Nobes, Mao Ye. Experimental investigation of fluid flow around a porous cube for Reynolds numbers of 400–1400. Chemical Engineering Science[J]. 2023, 第 4 作者269: http://dx.doi.org/10.1016/j.ces.2022.118443.
[4] Liang, Jinqiang, Liu, Danzhu, Xu, Shuliang, Ye, Mao. Modeling and analysis of air combustion and steam regeneration in MTO processes. Chinese Journal of Chemical Engineering[J]. 2023, 第 3 作者  通讯作者  
[5] Ma, Likun, Kashanj, Sina, Xu, Shuliang, Zhou, Jibin, Nobes, David S, Ye, Mao. Flow Reconstruction and Prediction Based on Small Particle Image Velocimetry Experimental Datasets with Convolutional Neural Networks. INDUSTRIAL ＆ ENGINEERING CHEMISTRY RESEARCH[J]. 2022, 第 3 作者61(24): 8504-8519, http://dx.doi.org/10.1021/acs.iecr.1c04704.
[6] Ma, Likun, Guo, Qiang, Li, Xue, Xu, Shuliang, Zhou, Jibin, Ye, Mao, Liu, Zhongmin. Drag correlations for flow past monodisperse arrays of spheres and porous spheres based on symbolic regression: Effects of permeability. Chemical Engineering Journal[J]. 2022, 第 4 作者445: http://dx.doi.org/10.1016/j.cej.2022.136653.
[7] Guo, Qiang, Bordbar, Alireza, Ma, Likun, Yu, Yaxiong, Xu, Shuliang, Boyce, Christopher M, Ye, Mao. A CFD-DEM study of the solid-like and fluid-like states in the homogeneous fluidization regime of Geldart A particles. AIChE Journal[J]. 2022, 第 5 作者68(1): http://dx.doi.org/10.1002/aic.17420.
[8] 梁金强, 刘丹竹, 徐庶亮, 叶茂, 刘中民. “双碳”目标下能源安全定量评价方法. 化工进展[J]. 2022, 第 3 作者41(3): 1622-1633, http://lib.cqvip.com/Qikan/Article/Detail?id=7106850851.
[9] Ma, Likun, Xu, Shuliang, Li, Xue, Guo, Qiang, Gao, Deyang, Ding, Ya, Ye, Mao, Liu, Zhongmin. Particle tracking velocimetry of porous sphere settling under gravity: Preparation of the model porous particle and measurement of drag coefficients. Powder Technology[J]. 2020, 第 2 作者360: 241-252, http://dx.doi.org/10.1016/j.powtec.2019.09.058.
[10] 张玉黎, 徐庶亮, 叶茂. 甲醇甲苯烷基化流化床反应器的数值模拟. 化工进展[J]. 2020, 第 2 作者39(12): 5057-5065, http://lib.cqvip.com/Qikan/Article/Detail?id=7103382239.
[11] Yiming Niu, Xing Huang, Yongzhao Wang, Ming Xu, Junnan Chen, Shuliang Xu, MarcGeorg Willinger, Wei Zhang, Min Wei, Bingsen Zhang. Manipulating interstitial carbon atoms in the nickel octahedral site for highly efficient hydrogenation of alkyne. NATURE COMMUNICATIONS[J]. 2020, 第 6 作者11(1): 1-9, Springer_JournalArticle.
[12] 于政锡, 徐庶亮, 张涛, 叶茂, 刘中民. 对二甲苯生产技术研究进展及发展趋势. 化工进展[J]. 2020, 第 2 作者39(12): 4984-4992, http://lib.cqvip.com/Qikan/Article/Detail?id=7103382232.
[13] 叶茂, 朱文良, 徐庶亮, 刘中民. 关于煤化工与石油化工的协调发展. 中国科学院院刊[J]. 2019, 第 3 作者417-425, http://lib.cqvip.com/Qikan/Article/Detail?id=75898988504849574852484856.
[14] Gao, Shushu, Xu, Shutao, Wei, Yingxu, Qiao, Qinglong, Xu, Zhaochao, Wu, Xinqiang, Zhang, Mozhi, He, Yanli, Xu, Shuliang, Liu, Zhongmin. Insight into the deactivation mode of methanol-to-olefins conversion over SAPO-34: Coke, diffusion, and acidic site accessibility. JOURNAL OF CATALYSIS[J]. 2018, 第 9 作者367: 306-314, http://dx.doi.org/10.1016/j.jcat.2018.09.010.
[15] Wu, Xinqiang, Xu, Shutao, Wei, Yingxu, Zhang, Wenna, Huang, Jindou, Xu, Shuliang, He, Yanli, Lin, Shanfan, Sun, Tantan, Liu, Zhongmin. Evolution of C-C Bond Formation in the Methanol-to-Olefins Process: From Direct Coupling to Autocatalysis. ACS CATALYSIS[J]. 2018, 第 6 作者8(8): 7356-7361, https://www.webofscience.com/wos/woscc/full-record/WOS:000441112400056.
[16] Zhou, Hui, Zhu, Wenliang, Shi, Lei, Liu, Hongchao, Liu, Shiping, Ni, Youming, Liu, Yong, He, Yanli, Xu, Shuliang, Li, Lina, Liu, Zhongmin. In situ DRIFT study of dimethyl ether carbonylation to methyl acetate on H-mordenite. JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL[J]. 2016, 第 9 作者417: 1-9, http://cas-ir.dicp.ac.cn/handle/321008/170776.
[17] Yuan, Danhua, He, Dawei, Xu, Shutao, Song, Zhijia, Zhang, Mozhi, Wei, Yingxu, He, Yanli, Xu, Shuliang, Liu, Zhongmin, Xu, Yunpeng. Imidazolium-based ionic liquids as novel organic SDA to synthesize high-silica Y zeolite. MICROPOROUS AND MESOPOROUS MATERIALS[J]. 2015, 第 8 作者204: 1-7, http://dx.doi.org/10.1016/j.micromeso.2014.10.049.
[18] 王全义, 魏迎旭, 徐舒涛, 张默之, 孟霜鹤, 樊栋, 齐越, 李金哲, 于政锡, 袁翠峪, 何艳丽, 徐庶亮, 陈景润, 王金棒, 苏宝连, 刘中民. 以一种新型Gemini表面活性剂作为介孔模板剂通过转晶过程合成介孔ZSM-5分子筛. 催化学报[J]. 2014, 第 12 作者35(10): 1727-1739, http://lib.cqvip.com/Qikan/Article/Detail?id=662797526.
[19] Yuan, Danhua, Xu, Shutao, Zhang, Mozhi, Wei, Yingxu, Dong, Xinglong, He, Yanli, Xu, Shuliang, Liu, Zhongmin, Xu, Yunpeng. Synthesis of ZSM-2 nanocrystals at ambient temperature. MICROPOROUS AND MESOPOROUS MATERIALS[J]. 2014, 第 7 作者185: 149-156, http://dx.doi.org/10.1016/j.micromeso.2013.11.010.
[20] Wang, Quanyi, Xu, Shutao, Chen, Jingrun, Wei, Yingxu, Li, Jinzhe, Fan, Dong, Yu, Zhengxi, Qi, Yue, He, Yanli, Xu, Shuliang, Yuan, Cuiyu, Zhou, You, Wang, Jinbang, Zhang, Mozhi, Su, Baolian, Liu, Zhongmin. Synthesis of mesoporous ZSM-5 catalysts using different mesogenous templates and their application in methanol conversion for enhanced catalyst lifespan. RSCADVANCES[J]. 2014, 第 10 作者4(41): 21479-21491, http://cas-ir.dicp.ac.cn/handle/321008/145610.
[21] Wang, Quanyi, Wei, Yingxu, Xu, Shutao, Zhang, Mozhi, Meng, Shuanghe, Fan, Dong, Qi, Yue, Li, Jinzhe, Yu, Zhengxi, Yuan, Cuiyu, He, Yanli, Xu, Shuliang, Chen, Jingrun, Wang, Jinbang, Su, Baolian, Liu, Zhongmin. Synthesis of mesoporous ZSM-5 using a new gemini surfactant as a mesoporous directing agent: A crystallization transformation process. CHINESE JOURNAL OF CATALYSIS[J]. 2014, 第 12 作者35(10): 1727-1739, http://dx.doi.org/10.1016/S1872-2067(14)60128-5.
[22] Chen, Jingrun, Li, Jinzhe, Yuan, Cuiyu, Xu, Shutao, Wei, Yingxu, Wang, Quanyi, Zhou, You, Wang, Jinbang, Zhang, Mozhi, He, Yanli, Xu, Shuliang, Liu, Zhongmin. Elucidating the olefin formation mechanism in the methanol to olefin reaction over AlPO-18 and SAPO-18. CATALYSIS SCIENCE & TECHNOLOGY[J]. 2014, 第 11 作者4(9): 3268-3277, http://cas-ir.dicp.ac.cn/handle/321008/145564.
[23] Xu Shuliang, Chu Wenling, Yang Weishen. The Effect of Preparation Procedure on the Performance of Pd-SiW12/SiO2 Catalysts for the Direct Oxidation of Ethylene to Acetic Acid. CHINESE JOURNAL OF CATALYSIS[J]. 2010, 第 1 作者31(11): 1342-1346, http://dx.doi.org/10.1016/S1872-2067(10)60123-4.
[24] 徐庶亮, 楚文玲, 杨维慎. 制备过程对Pd-SiW_（12）/SiO_2催化剂在乙烯选择氧化制乙酸反应中催化性能的影响. 催化学报[J]. 2010, 第 1 作者31(11): 1342-1346, http://lib.cqvip.com/Qikan/Article/Detail?id=36010828.
[25] Wang, Lixia, Xu, Shuliang, Chu, Wenling, Yang, Weishen. Effect of Pd loading and precursor on the catalytic performance of Pd/WO3-ZrO2 catalysts for selective oxidation of ethylene. CATALYSIS TODAY[J]. 2010, 第 2 作者149(1-2): 163-166, http://dx.doi.org/10.1016/j.cattod.2009.02.041.
[26] Xu Shuliang, Wang Lixia, Chu Wenling, Yang Weishen. Effect of Pore Structure of SiO2 on Catalytic Performance of Pd-SiW12/SiO2 for Direct Oxidation of Ethylene to Acetic Acid. CHINESE JOURNAL OF CATALYSIS[J]. 2009, 第 1 作者  通讯作者  30(10): 976-980, http://159.226.238.44/handle/321008/141499.
[27] 王丽霞, 徐庶亮, 楚文玲, 杨维慎. 贵金属对NM/WO3-ZrO2（NM=Ru，Rh和Pd）催化乙烯直接氧化制乙酸反应的影响（英文）. 催化学报[J]. 2009, 第 2 作者30(12): 1281-1286, http://lib.cqvip.com/Qikan/Article/Detail?id=32609421.
[28] 徐庶亮, 王丽霞, 楚文玲, 杨维慎. Pd-SiW12/SiO2 催化乙烯气相直接氧化制乙酸：SiO2 孔结构的影响. 催化学报[J]. 2009, 第 1 作者30(10): 976-980, http://lib.cqvip.com/Qikan/Article/Detail?id=32092158.
[29] Wang Lixia, Xu Shuliang, Chu Wenling, Yang Weishen. Influence of Noble Metals on the Direct Oxidation of Ethylene to Acetic Acid over NM/WO3-ZrO2 (NM = Ru, Rh, and Pd) Catalysts. CHINESE JOURNAL OF CATALYSIS[J]. 2009, 第 2 作者30(12): 1281-1286, http://dx.doi.org/10.1016/S1872-2067(08)60144-8.
[30] Xu, Shuliang, Wang, Lixia, Chu, Wenling, Yang, Weishen. Catalytic oxidation of ethylene to acetic acid on Pd-HPA/SiO2 catalysts with different heteropoly acids. REACTION KINETICS AND CATALYSIS LETTERS[J]. 2009, 第 1 作者98(1): 107-115, http://dx.doi.org/10.1007/s11144-009-0074-5.
[31] 王丽霞, 徐庶亮, 楚文玲, 杨维慎. Influence of Noble Metals on the Direct Oxidation of Ethylene to Acetic Acid over NM/WO3-ZrO2 (NM = Ru; Rh; and Pd) Catalysts. 催化学报[J]. 2009, 第 2 作者30(12): 1281-1286, http://159.226.238.44/handle/321008/102987.
[32] 楚文玲, 杨维慎, 王丽霞, 徐庶亮. Pd/WO3-ZrO2催化剂的结构对乙烯直接氧化制乙酸的影响. 催化学报[J]. 2009, 第 4 作者30(9): 864-872, http://lib.cqvip.com/Qikan/Article/Detail?id=31916399.
[33] Wang Lixia, Xu Shuliang, Chu Wenling, Yang Weishen. Effect of Structure of Pd/WO3-ZrO2 Catalyst on Its Activity for Direct Oxidation of Ethylene to Acetic Acid. CHINESE JOURNAL OF CATALYSIS[J]. 2009, 第 2 作者30(9): 864-872, http://dx.doi.org/10.1016/S1872-2067(08)60130-8.
[34] Xu, Shuliang, Wang, Lixia, Chu, Wenling, Yang, Weishen. Influence of Pd precursors on the catalytic performance of Pd-H4SiW12O40/SiO2 in the direct oxidation of ethylene to acetic acid. JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL[J]. 2009, 第 1 作者310(1-2): 138-143, http://dx.doi.org/10.1016/j.molcata.2009.06.008.
[35] 王丽霞, 楚文玲, 徐庶亮, 杨维慎. Pd/WO3–ZrO2 catalysts for direct oxidation of ethylene to acetic acid. A Pre-conference of the 14th Intenational Congress on Catalysis. 2008, 第 3 作者60/1, http://159.226.238.44/handle/321008/112982.
[36] 徐庶亮, 楚文玲, 王丽霞, 杨维慎. Influence of Pd precursors on the catalytic performance of Pd-H4SiW12O40/SiO2 in the direct oxidation of ethene to acetic acid. a pre-conference of the 14th international congress on catalysis. 2008, 第 1 作者258/1, http://159.226.238.44/handle/321008/112992.

（1） 多相流态化, 科学出版社, 2022-08, 第 其他 作者

   

（ 1 ） 甲醇转化限阈空间内环状有机物种的生成、催化机制及复合体系的主客体化学作用, 参与, 国家任务, 2013-01--2016-12
（ 2 ） SAPO-34分子筛催化甲醇及其衍生物转化初始C-H键活化和C-C键生成及自催化反应机制, 参与, 国家任务, 2018-01--2020-12
（ 3 ） 甲醇制芳烃工业示范, 参与, 国家任务, 2018-05--2021-04
（ 4 ） 能源安全战略研究, 负责人, 中国科学院计划, 2019-11--2020-12
（ 5 ） 工业反应器中多相流的动力学研究, 负责人, 地方任务, 2020-01--2022-04
（ 6 ） 等级孔催化材料的构筑理论和精准合成, 负责人, 国家任务, 2023-01--2027-12
（ 7 ） 新一代甲醇制烯烃技术及百万吨级工业示范, 参与, 中国科学院计划, 2018-04--2023-04
（ 8 ） 50万吨/年甲醇制丙烯流化床技术工业示范, 参与, 中国科学院计划, 2022-02--2027-02
（ 9 ） 宁东基地煤化工产业链延伸与产品耦合发展研究, 参与, 国家任务, 2020-01--2021-12

现指导学生

田宇  硕士研究生  085600-材料与化工