基本信息
何广智  男  博导  中国科学院生态环境研究中心
电子邮件: gzhhe@rcees.ac.cn
通信地址: 海淀区双清路18号
邮政编码:

招生信息

   
招生专业
083001-环境科学
招生方向
环境催化,大气污染控制

教育背景

2006-09--2011-06   中国科学院生态环境研究中心   博士
2002-09--2006-06   中国地质大学(北京)   学士

工作经历

   
工作简历
2023-01~现在, 中国科学院生态环境研究中心, 研究员
2018-04~2023-01,中国科学院生态环境研究中心, 副研究员
2011-07~2018-04,中国科学院生态环境研究中心, 助理研究员
2006-09~2011-06,中国科学院生态环境研究中心, 博士
2002-09~2006-06,中国地质大学(北京), 学士

教授课程

环境催化原理
气溶胶化学

专利与奖励

   
奖励信息
(1) 中国科学院青年创新促进会优秀会员, 院级, 2024
(2) 国家“万人计划”青年拔尖人才, , 国家级, 2022
(3) 中国科学院青年创新促进会会员, , 院级, 2019
(4) 中国科学院院长优秀奖, 院级, 2011
专利成果
( 1 ) 一种硫化钒钛催化剂及其制备方法和用途, 2019, 第 5 作者, 专利号: CN109174125A

出版信息

   
发表论文
(1) Spatial Distribution of Br��nsted Acid Sites Determines the Mobility of Reactive Cu Ions in the Cu-SSZ-13 Catalyst during the Selective Catalytic Reduction of NOx with NH3, Journal of the American Chemical Society, 2024, 
(2) Combined Experimental and Density Functional Theory Study on the Mechanism of the Selective Catalytic Reduction of NO with NH3 over Metal-Free Carbon-Based Catalysts, Environmental Science & Technology, 2024, 
(3) Unexpected Promotion Effect of H2O on the Selective Catalytic Reduction of NOx with NH3 over Cu-SSZ-39 Catalysts, Environmental Science & Technology, 2024, 
(4) Uncovering the Dinuclear Mechanism of NO2���Involved NH3���SCR over Supported V2O5/TiO2 Catalysts, Environmental Science & Technology, 2024, 
(5) Interface sites on vanadia-based catalysts are highly active for NOx removal under realistic conditions, JOURNAL OF ENVIRONMENTAL SCIENCES, 2024, 第 2 作者  通讯作者
(6) A review on the heterogeneous oxidation of SO 2 on solid atmospheric particles: Implications for sulfate formation in haze chemistry, CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY, 2023, 第 4 作者
(7) A review on the heterogeneous oxidation of SO2 on solid atmospheric particles: Implications for sulfate formation in haze chemistry, CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY, 2023, 第 4 作者
(8) Mechanistic Insight into the Promotion of the Low-Temperature NH3-Selective Catalytic Reduction Activity over MnxCe1-xOy Catalysts: A Combined Experimental and Density Functional Theory Study, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 第 3 作者  通讯作者
(9) Unveiling the Origin of Selectivity in the Selective Catalytic Reduction of NO with NH3 over Oxide Catalysts, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 第 3 作者  通讯作者
(10) Atmospheric heterogeneous reactions on soot: A review, FUNDAMENTAL RESEARCH, 2023, 第 2 作者
(11) Neglected but Efficient Electron Utilization Driven by Biochar- Coactivated Phenols and Peroxydisulfate: Polyphenol Accumulation Rather than Mineralization, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 第 4 作者
(12) Dehydration-enhanced ion-pore interactions dominate anion transport and selectivity in nanochannels, SCIENCE ADVANCES, 2023, 第 6 作者
(13) Strikingly distinctive NH3-SCR behavior over Cu-SSZ-13 in the presence of NO2, NATURE COMMUNICATIONS, 2022, 第 2 作者  通讯作者
(14) Si/Al Ratio Determines the SCR Performance of Cu-SSZ-13 Catalysts in the Presence of NO2, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2022, 第 8 作者
(15) Layered Double Hydroxide Catalysts for Ozone Decomposition: The Synergic Role of M2+ and M3+, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2022, 第 4 作者  通讯作者
(16) Effect of Hydroxyl Groups on Metal Anchoring and Formaldehyde Oxidation Performance of Pt/Al2O3, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2022, 第 2 作者
(17) Promotion of the selective catalytic reduction of NOx with NH3 over microporous Cu-SSZ-13 by H2O and OH groups at low temperatures: a density functional theory study, CATALYSIS SCIENCE & TECHNOLOGY, 2022, 第 2 作者  通讯作者
(18) Generation and Release of OH Radicals from the Reaction of H2O with O2 over Soot, Angewandte Chemie International Edition, 2022, 第 1 作者
(19) A robust H-transfer redox mechanism determines the high-efficiency catalytic performance of layered double hydroxides, APPLIED CATALYSIS B-ENVIRONMENTAL, 2021, 第 3 作者  通讯作者
(20) Theory and practice of metal oxide catalyst design for the selective catalytic reduction of NOx with NH3, CATALYSIS TODAY, 2021, 第 4 作者
(21) Introducing tin to develop ternary metal oxides with excellent hydrothermal stability for NH3 selective catalytic reduction of NOx, APPLIED CATALYSIS B-ENVIRONMENTAL, 2021, 第 2 作者
(22) Superior Oxidative Dehydrogenation Performance toward NH3 Determines the Excellent Low-Temperature NH3-SCR Activity of Mn-Based Catalysts, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2021, 第 1 作者
(23) Layered Double Hydroxide Catalysts for Ozone Decomposition: The Synergic Role of M2+ and M3+, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2021, 第 4 作者  通讯作者
(24) Reaction Pathways of the Selective Catalytic Reduction of NO with NH3 on the alpha-Fe2O3(012) Surface: a Combined Experimental and DFT Study, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2021, 第 2 作者  通讯作者
(25) Photochemical Aging of Atmospheric Fine Particles as a Potential Source for Gas-Phase Hydrogen Peroxide, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2021, 第 4 作者
(26) Adsorption-Induced Active Vanadium Species Facilitate Excellent Performance in Low-Temperature Catalytic NOx Abatement, JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2021, 第 7 作者
(27) Tuning the fill percentage in the hydrothermal synthesis process to increase catalyst performance for ozone decomposition, Tuning the fill percentage in the hydrothermal synthesis process to increase catalyst performance for ozone decomposition, JOURNAL OF ENVIRONMENTAL SCIENCES, 2020, 第 4 作者
(28) Improving the catalytic performance of ozone decomposition over Pd-Ce-OMS-2 catalysts under harsh conditions, CATALYSIS SCIENCE & TECHNOLOGY, 2020, 第 4 作者
(29) Identification of a Facile Pathway for Dioxymethylene Conversion to Formate Catalyzed by Surface Hydroxyl on TiO2-Based Catalyst, ACS CATALYSIS, 2020, 第 2 作者
(30) The way to enhance the thermal stability of V2O5-based catalysts for NH3-SCR, CATALYSIS TODAY, 2020, 第 4 作者
(31) In Situ Surface-Enhanced Raman Spectroscopic Evidence on the Origin of Selectivity in CO2 Electrocatalytic Reduction, ACS NANO, 2020, 第 7 作者
(32) Water Promotes the Oxidation of SO2 by O-2 over Carbonaceous Aerosols, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2020, 第 1 作者  通讯作者
(33) Atomic-scale insights into zeolite-based catalysis in N2O decomposition, SCIENCE OF THE TOTAL ENVIRONMENT, 2019, 第 1 作者
(34) Insights into the Activation Effect of H-2 Pretreatment on Ag/Al2O3 Catalyst for the Selective Oxidation of Ammonia, ACS CATALYSIS, 2019, 第 2 作者
(35) Insights into the activation effect of H2 pretreatment on Ag/Al2O3 catalyst for the selective catalytic oxidation of ammonia, ACS Catal., 2019, 
(36) Experimental and DFT study of the adsorption of N2O on transition ion-exchanged ZSM-5, CATALYSIS TODAY, 2019, 第 2 作者
(37) Oxygen vacancies induced by transition metal doping in ������MnO2 for highly efficient ozone decomposition, Environ. Sci. Technol., 2018, 
(38) Nanosize effect of al2o3 in ag/al2o3 catalyst for the selective catalytic oxidation of ammonia, ACS CATALYSIS, 2018, 第 3 作者
(39) Role of carbonaceous aerosols in catalyzing sulfate formation, ACS CATALYSIS, 2018, 第 1 作者
(40) Polymeric vanadyl species determine the low-temperature activity of V-based catalysts for the SCR of NOx with NH3, SCIENCE ADVANCES, 2018, 第 1 作者
(41) Effects of no2 addition on the nh3-scr over small-pore cu-ssz-13 zeolites with varying cu loadings, JOURNAL OF PHYSICAL CHEMISTRY C, 2018, 第 3 作者
(42) Oxygen vacancies induced by transition metal doping in gamma-mno2 for highly efficient ozone decomposition, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 第 4 作者
(43) Synergistic Effect of TiO2-SiO2 in Ag/Si-Ti Catalyst for the Selective Catalytic Oxidation of Ammonia, INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2018, 第 3 作者
(44) Specific Role of Potassium in Promoting Ag/Al2O3 for Catalytic Oxidation of Formaldehyde at Low Temperature, JOURNAL OF PHYSICAL CHEMISTRY C, 2018, 第 3 作者
(45) Structure-activity relationship of surface hydroxyl groups during no2 adsorption and transformation on tio2 nanoparticles, ENVIRONMENTAL SCIENCE-NANO, 2017, 第 4 作者
(46) Remarkable synergistic effect between {001} facets and surface F ions promoting hole migration on anatase TiO2, APPLIEDCATALYSISBENVIRONMENTAL, 2017, 第 4 作者
(47) An alumina-supported silver catalyst with high water tolerance for H2 assisted C3H6-SCR of NOx, APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 第 3 作者
(48) Selective h2o2 conversion to hydroxyl radicals in the electron-rich area of hydroxylated c-g-c3n4/ cuco-al2o3, JOURNAL OF MATERIALS CHEMISTRY A, 2017, 第 3 作者
(49) DFT studies on the heterogeneous oxidation of SO2 by oxygen functional groups on graphene, PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2016, 第 1 作者
(50) Layered sphere-shaped TiO2 capped with gold nanoparticles on structural defects and their catalysis of formaldehyde oxidation, JOURNAL OF ENVIRONMENTAL SCIENCES, 2016, 第 3 作者
(51) Layered sphere-shaped TiO2 capped with gold nanoparticles on structural defects and their catalysis of formaldehyde oxidation, JOURNAL OF ENVIRONMENTAL SCIENCES-CHINA, 2016, 第 3 作者
(52) Nanobubbles at Hydrophilic Particle-Water Interfaces, LANGMUIR, 2016, 第 2 作者
(53) Binding mechanism of arsenate on rutile (1 1 0) and (0 0 1) planes studied using grazing-incidence EXAFS measurement and DFT calculation, CHEMOSPHERE, 2015, 第 2 作者
(54) Molecular dynamics simulations of structural transformation of perfluorooctane sulfonate (PFOS) at water/rutile interfaces, CHEMOSPHERE, 2015, 第 1 作者  通讯作者
(55) Simultaneous Multifunctional Sorption of PFOS and Cr(VI) on Activated Carbon Prepared by One-Step Microwave Activation, WATER AIR AND SOIL POLLUTION, 2015, 第 4 作者
(56) Structure and stability of arsenate adsorbed on ��-Al2O3 single-crystal surfaces investigated using grazing-incidence EXAFS measurement and DFT calculation, CHEMICAL GEOLOGY, 2014, 第 2 作者
(57) Structure and stability of arsenate adsorbed on alpha-Al2O3 single-crystal surfaces investigated using grazing-incidence EXAFS measurement and DFT calculation, CHEMICAL GEOLOGY, 2014, 第 2 作者
(58) Assembling structures and dynamics properties of perfluorooctane sulfonate (PFOS) at water���titanium oxide interfaces, JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2013, 第 1 作者
(59) Perfluorooctane sulfonate removal by nanofiltration membrane the role of calcium ions, CHEMICAL ENGINEERING JOURNAL, 2013, 第 3 作者
(60) PFOS在锐钛型TiO2表面吸附行为的理论研究, Theoretical Studies on Adsorption of PFOS on Anatase TiO2 Surfaces, 高等学校化学学报, 2013, 第 2 作者
(61) Theoretical Studies on Adsorption of PFOS on Anatase TiO2 Surfaces, CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE, 2013, 第 2 作者  通讯作者
(62) XANES analysis of spectral properties and structures of arsenate adsorption on TiO2 surfaces, JOURNAL OF SYNCHROTRON RADIATION, 2012, 第 1 作者
(63) XANES analysis of spectral properties and structures of arsenate adsorption on TiO2 surfaces, INSTRUMENTS & INSTRUMENTATION; OPTICS; PHYSICS, 2012, 第 1 作者
(64) XAFS study of starch-stabilized magnetite nanoparticles and surface speciation of arsenate, ENVIRONMENTAL POLLUTION, 2011, 第 4 作者
(65) Coordination Structure of Adsorbed Zn(II) at Water-TiO2 Interfaces, ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2011, 第 1 作者
(66) Studies on the reaction pathway of arsenate adsorption at water���TiO2 interfaces using density functional theory, JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2011, 第 1 作者
(67) Quantitative XANES Studies on Metastable Equilibrium Adsorption of Arsenate on TiO2 Surfaces, JOURNAL OF PHYSICAL CHEMISTRY C, 2009, 第 1 作者
(68) Combined DFT and IR evidence on metastable-equilibrium adsorption of arsenate on TiO2 surfaces, JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2009, 第 2 作者
(69) Zn(Ⅱ)在TiO2表面上的微观吸附模式研究, Study of Microscopic Adsorption Modes of Zn( ��� ) on TiO2 Surface, 高等学校化学学报, 2009, 第 6 作者
(70) As(Ⅴ)在TiO_2表面的吸附机理, Mechanism of Arsenate (���) Adsorption on TiO_2 Surfaces, 物理化学学报, 2009, 第 2 作者
(71) Zn(II)在TiO2表面上的微观吸附模式研究, 高等学校化学学报, 2009, 第 1 作者
(72) Influence of pH on Initial Concentration Effect of Arsenate Adsorption on TiO2 Surfaces: Thermodynamic, DFT, and EXAFS Interpretations, JOURNAL OF PHYSICAL CHEMISTRY C, 2009, 第 1 作者
(73) 用EXAFS研究pH对Zn(II)-TiO2体系吸附和微观构型的影响, 高等学校化学学报, 2009, 第 1 作者
(74) Mechanism of Arsenate (V) Adsorption on TiO2 Surfaces, ACTA PHYSICO-CHIMICA SINICA, 2009, 第 2 作者
(75) 用EXAFS研究pH对Zn(Ⅱ)-TiO2体系吸附和微观构型的影响, EXAFS Studies of pH Effects on Adsorption and Microscopic Strutures of Zn( ��� ) onto TiO2, 高等学校化学学报, 2009, 第 2 作者
(76) As(V)在TiO2表面的吸附机理, Mechanism of Arsenate (���) Adsorption on TiO2 Surfaces, 物理化学学报, 2009, 第 2 作者
(77) 分子环境科学与亚稳平衡吸附理论研究进展, Molecular environmental science and metastable-equilibrium adsorption theory, 物理, 2009, 第 2 作者
(78) EXAFS Studies of pH Effects on Adsorption and Microscopic Strutures of Zn( II ) onto TiO2, CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE, 2009, 第 3 作者
(79) EXAFS studies on adsorption irreversibility of Zn(II) on TiO 2: Temperature dependence, JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2008, 第 7 作者
(80) 用延展X射线精细结构吸收光谱研究Zn(Ⅱ)-TiO2体系的颗粒物浓度效应和吸附可逆性, EXAFS studies on particle concentration effect and adsorption reversibility of Zn( ��� ) onto anatase TiO2, 核技术, 2007, 第 5 作者
(81) 温度对Zn(II)-TiO_2体系吸附可逆性的影响, 物理化学学报, 2007, 第 5 作者
(82) 温度对Zn(Ⅱ)-TiO2体系吸附可逆性的影响, Temperature Effects on Adsorption-Desorption Irreversibility of Zn(���) onto Anatase, 物理化学学报, 2007, 第 5 作者
(83) 用延展X射线精细结构吸收光谱研究Zn(II)-TiO2体系的颗粒物浓度效应和吸附可逆性, 核技术, 2007, 第 1 作者
(84) Interface sites on vanadia-based catalysts are highly active for NOx removal under realistic conditions, JOURNAL OF ENVIRONMENTAL SCIENCES, 第 2 作者
发表著作
Advances in Interfacial Adsorption Thermodynamics: Metastable-Equilibrium Adsorption (MEA) Theory, InTech, 2011-11, 第 2 作者

科研活动

   
科研项目
( 1 ) 中国科学院青年创新促进会优秀会员人才专项经费, 负责人, 中国科学院计划, 2024-01--2026-12
( 2 ) 新型燃料动力船舶尾气超低排放控制技术及装备研发, 负责人, 国家任务, 2023-12--2027-11
( 3 ) 钒基NH3-SCR催化剂活性位结构调控及耦合效应机制研究, 负责人, 国家任务, 2023-01--2026-12
( 4 ) 国家“万人计划”青年拔尖人才, 负责人, 国家任务, 2022-09--2025-09
( 5 ) 大气霾化学基础科学中心项目, 参与, 国家任务, 2022-01--2026-12
( 6 ) 中国科学院青年创新促进会会员人才专项经费, 负责人, 中国科学院计划, 2019-01--2022-12
( 7 ) 黑碳活化O2及催化氧化SO2生成硫酸盐二次粒子作用机理研究, 负责人, 国家任务, 2018-01--2021-12
( 8 ) 柴油车NOx后处理关键技术, 参与, 国家任务, 2017-07--2020-12
( 9 ) 柴油车整车排放控制集成及应用示范, 参与, 国家任务, 2017-07--2020-12
( 10 ) 柴油车尾气净化用高性能NH3-SCR催化剂基础研究, 参与, 国家任务, 2017-01--2021-12
( 11 ) 典型PFCs污染物与水/固界面作用机理及结构的研究, 负责人, 国家任务, 2013-01--2015-12